Results 191 to 200 of about 125,899 (235)

Ferrocene‐Based Self‐Assembled Monolayers Enable Ultra‐High Specific Detectivity in Perovskite Photodetectors

open access: yesAdvanced Materials, EarlyView.
We report perovskite photodetectors with record specific detectivities exceeding 1013 Jones with a novel molecular design strategy to functionalize self‐assembled monolayers (SAMs) with ferrocene (Fc) derivatives. Fc‐SAM‐based devices also exhibit strong operational stability and enable data transmission rates exceeding 1 Mbps in a LiFi system ...
Edoardo Angela   +10 more
wiley   +1 more source

Interface‐Mediated Catalysis for Improved Hydrogen Storage in Reactive Hydride Composites

open access: yesAdvanced Materials, EarlyView.
Catalyst–hydride interfaces are engineered in Co@C‐ and Ni@C‐modified 2LiH + MgB2 reactive hydride composites to accelerate hydrogen uptake and release. Multiscale scattering, in‐situ synchrotron radiation powder x‐ray diffraction and density functional theory calculations reveal the structural and electronic origin of the catalytic enhancement ...
Yuanyuan Shang   +12 more
wiley   +1 more source

Plasmon‐Enhanced Second‐Harmonic Generation in Atomically Thin Crystalline Silver Nanostructures

open access: yesAdvanced Materials, EarlyView.
Atomically thin crystalline silver films combine vertical quantum confinement with lateral plasmonic field enhancement to boost second‐harmonic generation. Nanoribbon and nanotriangle arrays enable geometry‐tunable infrared plasmon resonances, producing strong SHG from deeply subwavelength metallic volumes compatible with silicon‐based nanophotonics ...
Saad Abdullah   +10 more
wiley   +1 more source

Phase‐Engineered MoS2 Quantum Monolayer Catalysts

open access: yesAdvanced Materials, EarlyView.
A new type of catalyst model—phase‐engineered MoS2 quantum‐monolayer catalyst (∼0.8 nm thick, < 6 nm in the lateral size; switchable freely among metallic 1T, semiconducting 2H, and a hybrid phase of metallic‐semiconducting 1T‐2H)—is reported. It can efficiently and stably drive photochemical H2, syngas and ammonia synthesis as a catalyst or co ...
Ruijie Yang   +12 more
wiley   +1 more source

Ionic Cocrystal Programming of Spatial Ionic Organization in Carbon Nitrides Enables Highly Efficient H2O2 Photosynthesis

open access: yesAdvanced Materials, EarlyView.
Ionic cocrystal‐programmed ionic organization establishes a general strategy for electrostatic programming in polymeric photocatalysts. ABSTRACT Controlling the spatial organization of ions in polymeric photocatalysts remains a fundamental challenge for optimizing charge transport and catalytic selectivity in solar‐driven hydrogen peroxide (H2O2 ...
Anna Lo Presti   +6 more
wiley   +1 more source

Highly Sensitive Broadband Photodetectors Based on Donor–Acceptor 2D Conjugated Coordination Polymers

open access: yesAdvanced Materials, EarlyView.
Donor–acceptor molecular design and chemical vapor deposition growth enable the two‐dimensional nickel‐tetraaminobenzoquinone films with strong broadband absorption and efficient charge separation. The resulting photodetectors exhibit a structured broadband response with a high responsivity of ∼3.1 A W−1 and a response time of ∼170 µs, which surpasses ...
Yunxu Chen   +14 more
wiley   +1 more source

Layered Spin‐Crossover Metal‐Organic Frameworks for Light‐Induced Control of Two‐Dimensional Quantum Materials

open access: yesAdvanced Materials, EarlyView.
Spin‐crossover metal‐organic frameworks (SCO‐MOFs) provide a route to control the electronic and magnetic properties of two‐dimensional quantum materials. By integrating a layered SCO‐MOFs with graphene, CrSBr, and NbSe2 nanodevices, thermally and light induced spin transitions induce strain that reversibly modulates charge transport, magnetic memory ...
Carla Boix‐Constant   +4 more
wiley   +1 more source

Synthesis of Bulk Superconducting LiNbO2 Crystals Through CaH2 Reduction

open access: yesAdvanced Materials, EarlyView.
CaH2 reduction reconstructively transforms insulating LiNbO3 single crystals into superconducting bulk LiNbO2 with a critical temperature of Tc = 14.4 K. Scanning electron microscopy reveals large‐volume, high‐yield phase conversion. Magnetization measurements demonstrate a robust ∼ 77% Meissner shielding fraction, establishing bulk superconductivity ...
Ryan Paxson   +19 more
wiley   +1 more source

Turning Nd‐Fe‐B Swarf Into High‐Value Bulk Feedstocks via Sustainable Hydrogen Plasma: From Rare‐Earth Oxides to Metals and Hydrides

open access: yesAdvanced Materials, EarlyView.
Oxidized Nd‐Fe‐B magnet swarf is transformed into valuable bulk feedstock through a single‐step hydrogen plasma process. The reaction converts complex rare‐earth‐containing waste into separated metallic, oxide, and hydride fractions without acid leaching.
Naritai Chimed   +9 more
wiley   +1 more source

Chiral Phonon–Driven Ultrafast Spin Currents in a Non‐Magnetic Ferroelectric

open access: yesAdvanced Materials, EarlyView.
Broadband terahertz emission spectroscopy shows signatures of ultrafast spin‐current generation in non‐magnetic ferroelectric β$\beta$’‐In2Se3${\rm In}_2{\rm Se}_3$. Reversal of the emitted field upon sample inversion and substitution of Pt with W indicates spin‐Hall‐mediated charge conversion, while polarization‐resolved measurements reveal ...
Thomas B. Gill   +16 more
wiley   +1 more source

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