Results 181 to 190 of about 41,428 (262)

Ultrafast, High‐Capacity Uranium Harvesting From Seawater via a Hierarchically Porous Polymer Electrode

open access: yesAdvanced Science, EarlyView.
A hierarchically porous AOPIM‐CNT electrode enables uranium harvesting from seawater via adsorption‐promoted electrodeposition. Rapid diffusion and selective adsorption are coupled with electrochemical crystallization and spontaneous detachment, creating a self‐refreshing process that sustains high‐capacity, continuous extraction from ultradilute ...
Zejun Song   +7 more
wiley   +1 more source

CO2‐to‐CO Electrolysis in Pure Water at Ampere‐Level Current Density and 1000 h Stability via a Rapid‐Transport Fixed‐Charge Interface

open access: yesAdvanced Science, EarlyView.
CO2 reduction in pure water is enabled by a rapid‐transport fixed‐charge interface that couples nanochannels with a cationic microenvironment. This design eliminates the mass transport plateau, stabilizes key reaction intermediates, and suppresses the hydrogen evolution reaction, ultimately achieving ampere‐level current densities and stable operation ...
Qiqi Wan   +8 more
wiley   +1 more source

Giant Conductivity Modulation and Chemical Neuromodulation via Proton‐Electron Coupling in a Hydrogen‐Bonded Coordination Polymer

open access: yesAdvanced Science, EarlyView.
A “de‐doping” strategy positions mixed protonic–electronic conductors (MPECs) as adaptive neuromorphic platforms with dynamically tunable transport. Co‐BAND achieves giant conductivity modulation (>106) and chemically tunable synaptic plasticity. Analogous to biological neuromodulation, solvent vapors dynamically reprogram the device's learning rules ...
Kwangmin Park   +10 more
wiley   +1 more source

Heterointerface Engineering of Bismuth Nanosheets/Nitrogen‐Doped Carbon Nanoleaves Enables High‑Performance Electrochemical Dechlorination

open access: yesAdvanced Science, EarlyView.
Bismuth nanosheets integrated with nitrogen‐doped carbon nanoleaves are constructed via a 2D‐on‐2D heterointerface engineering strategy. The resulting BiNS/NCL electrode delivers high chloride adsorption capacity, fast kinetics, and stable cyclability. A built‐in electric field at the heterointerface promotes chloride electrosorption and stabilizes the
Bohan Liu   +11 more
wiley   +1 more source

Reaction‐Induced Reversible Reconstruction Enhanced Ni‐MgO/CaO Dual Functional Material for Stable CO2 Capture and In Situ Conversion

open access: yesAdvanced Science, EarlyView.
A highly dispersed NiO‐MgO solid solution (MgxNi1‐xO) is created in a hierarchically porous Ca‐based matrix to protect Ni and CaO nanoparticles against carbon deposition and sintering. Owing to the reversible reconstruction of MgxNi1‐xO, this superior structure is self‐regenerative in the calcium looping dry reforming of methane process, thereby ...
Hao Xu   +5 more
wiley   +1 more source

N‐Doping Activated Presodiation Enhances Sodium‐Ion Provision in Hard Carbon Anodes

open access: yesAdvanced Science, EarlyView.
Introducing pyrrolic‐N sites enables efficient presodiation and stronger PF6− capture, thus pre ‐ forming a robust inorganic‐rich SEI layer in hard carbon anodes. ABSTRACT Hard carbon (HC) is considered the most promising anode material for commercial sodium‐ion batteries (SIBs), yet it still faces critical challenges such as low initial Coulombic ...
Hua Lin   +8 more
wiley   +1 more source

Spatially Separated Redox Centers in One‐Dimensional Sp2‐Carbon Covalent Organic Frameworks Enable Synergistic Photocatalytic Palladium Recovery and Bisphenol A Mineralization

open access: yesAdvanced Science, EarlyView.
A one‐dimensional sp2‐carbon covalent organic framework with spatially segregated redox centers integrates a dual photosensitizing system and a cationic interface for synergistic photocatalysis. The material achieves exceptional palladium recovery (1749 mg g−1) and bisphenol A mineralization (0.1710 min−1) without sacrificial agents, demonstrating ...
Yi‐Ru Chen   +9 more
wiley   +1 more source

Lunar‐Based Photothermal CO2 Reduction Strategy: Self‐Evolving Transient Active Interface and Band Engineering

open access: yesAdvanced Science, EarlyView.
A self‐evolving Pd/Ov‐FeTiO3 photothermal catalyst, inspired by lunar soil, enables efficient extraterrestrial CO2 conversion. The formation of transient active interfaces and oxygen vacancies extends light absorption to the infrared range and optimizes electron transfer.
Yahang Wang   +11 more
wiley   +1 more source

Heterojunction‐Engineered Mass Spectrometry Platform for Deciphering Serum Metabolic Fingerprints in Diagnosis of Respiratory Diseases

open access: yesAdvanced Science, EarlyView.
Hollow Co3O4/TiO2 heterojunctions are engineered for high‐throughput laser desorption/ionization mass spectrometry. The built‐in electric field drives efficient charge separation and photothermal conversion, while the hierarchical mesoporous network enables robust salt and protein tolerance.
Junyu Chen   +8 more
wiley   +1 more source

Dipole‐Manipulated Built‐In Electric Field Enables Ultrafast Charge Separation in Perylene Diimide Polymers for Photoelectrochemical Water Splitting

open access: yesAdvanced Science, EarlyView.
Molecular dipole engineering in dendritic perylene diimide polymers through nitrogen‐rich heterocyclic linkers amplifies the built‐in electric field, enabling sub‐picosecond charge separation and efficient multi‐electron accumulation. This structure–dynamics–performance relationship establishes a versatile design strategy for high‐performance organic ...
Ying‐Xin Qiao   +11 more
wiley   +1 more source

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