Results 121 to 130 of about 980,173 (306)

Engineering Bilayer Tandem Catalysts on Si‐Based Photocathodes for High‐performance CO2 Reduction to Produce Methane

Advanced Materials, EarlyView.
A Cu/Ag‐Cu bilayer tandem catalyst is designed for a pyramid‐structured p‐Si photocathode, creating multiple and functionally distinct interfaces tailored to specific reaction steps and intermediate stabilization. This Cu/Ag‐Cu‐decorated p‐Si photocathode exhibits both high photocurrent and good selectivity for photoelectrochemical CO2 reduction to CH4.
Hao Wu, Shenghe Si, Haitao Wang, Changlai Wang, Rongchi Dai, Jianuo Li, Shohei Fukaya, Zhenhua Pan, Yujie Xiong, Noritaka Usami, Koyo Norinaga, Yasuyoshi Kurokawa, Suchada Sirisomboonchai, Dong Liu, Qian Wang   +14 more
wiley   +1 more source

High‐κ Perovskite‐Like Ternary Niobium Oxide Dielectrics for 2D Electronics

Advanced Materials, EarlyView.
High‐κ dielectrics are vital for scaled electronics. Here, a family of 2D high‐κ perovskite‐like ternary niobium oxides is synthesized via a molten salt‐assisted method. Their integration into FETs and logic gates reveals superior switching characteristics, providing a fresh material platform and new insights for the advancement of high‐performance 2D ...
Biao Zhang, Jianmiao Guo, Jianmin Yan, Jialiang Wang, Chao Yun, Guang Zeng, Jie Li, Cong Wang, Zhengdao Xie, Yanglong Hou, Yang Chai   +10 more
wiley   +1 more source

Superionic Amorphous Li2ZrCl6 and Li2HfCl6

Advanced Materials, EarlyView.
Amorphous Li2HfCl6 and L2ZrCl6 are shown to be promising solid‐state electrolytes with predicted ionic conductivities >20 mS·cm−1. Molecular dynamics simulations with machine‐learning force fields reveal that anion vibrations and flexible MCl6 octahedra soften the Li coordination cage and enhance mobility. Correlation between Li‐ion diffusivity and the
Shukai Yao, De‐en Jiang
wiley   +1 more source

On‐Surface Synthesis of Bismuth Monolayers through Ice‐Confined Redox Reactions

Advanced Materials, EarlyView.
We report an ice‐confined growth strategy for the synthesis of atomically thin 2D bismuth and related 2D metals. This approach involves rapid freezing of a BiCl3 aqueous solution on an aluminum foil using liquid nitrogen, which triggers interfacial redox reactions between the ice and the aluminum surface.
Zexiang He, Depeng Wang, Wentao Fan, Songlin Liu, Antonio Gaetano Ricciardulli, Haixia Zhong, Yiyong Mai, Paolo Samorì, Sheng Yang   +8 more
wiley   +1 more source

Entanglement asymmetry and symmetry defects in boundary conformal field theory

Journal of High Energy Physics
A state in a quantum system with a given global symmetry, G, can be sensitive to the presence of boundaries, which may either preserve or break this symmetry.
Yuya Kusuki, Sara Murciano, Hirosi Ooguri, Sridip Pal   +3 more
doaj   +1 more source

Designing Defect Structure and Interfacial Strain in an Epitaxial VN Bilayer Film by Tailoring N Concentration

Advanced Materials Interfaces, EarlyView.
The N concentration in an epitaxial VN bilayer is tailored from overstoichiometric V0.49N0.51 to understoichiometric V0.56N0.44. Based on ab initio, diffraction, and microscopy data, the overstoichiometric V0.49N0.51 layer contains V vacancies, N Frenkel pairs, and a high density of dislocations.
Marcus Hans, Damian M. Holzapfel, Zhuo Chen, Soheil Karimi Aghda, Michal Fečík, Daniel Primetzhofer, Zaoli Zhang, Jochen M. Schneider   +7 more
wiley   +1 more source

Investigating the Structural Factors Influencing the Magnetic Interaction between Individual Copper Spins in the CuCu4 Metallacrown Complex, from Its Bulk Form to Its Adsorption on Au(111)

Advanced Materials Interfaces, EarlyView.
The Cu(II)[12‐MCCu(II)N(Shi)‐4] metallacrown complex (CuCu4) is studied to examine how geometric transformations affect magnetic coupling between copper spins by using ultraviolet photoemission spectroscopy and DFT calculations for the bulk phase and CuCu4 adsorbed on Au(111). While adsorption minimally affects tDOS, exchange coupling constants between
Ariyan Tavakoli, Stefan Lach, Frederik Pütz, Dominic Stephan, Anne Lüpke, Dominik Laible, Siegfried Kaidisch, Andreas Windischbacher, Eva Rentschler, Peter Puschnig, Hans‐Christian Schneider, Christiane Ziegler   +11 more
wiley   +1 more source

Amido‐Amine Co(II) Precursor‐Based Atomic/Molecular Layer Deposition Processes for Cobalt‐Organic Thin Films and Their Thermal Conversion to CoO Thin Films

Advanced Materials Technologies, EarlyView.
Three new atomic/molecular layer deposition processes are developed for Co‐organic thin films using a promising all‐nitrogen‐coordinated cobalt precursor. The study examines film growth, reaction mechanisms, chemical stability, and decomposition pathways of the resulting films through extensive characterization techniques and DFT calculations ...
Topias Jussila, Jorit Obenlüneschloß, Ji Liu, Olga Partanen, Sami Vasala, Detlef Rogalla, Pieter Glatzel, Michael Nolan, Anjana Devi, Maarit Karppinen   +9 more
wiley   +1 more source

Incorporating Si into Sb2Se3: Tailoring Optical Phase Change Materials via Nanocomposites

Advanced Optical Materials, EarlyView.
We study the structural, optical, and thermal effects of adding silicon to Sb2Se3 and demonstrate that the as‐deposited solid solution phase segregates after electro‐thermal switching, creating a nanocomposite with effective‐medium properties and a phase‐change response.
Chih‐Yu Lee, Yi‐Siou Huang, Felix Adams, Chuanyu Lian, Hongyi Sun, Jie Zhao, Zichao Ye, Nathan Youngblood, Juejun Hu, Leslie H Allen, Yifei Mo, Ichiro Takeuchi, Carlos A Ríos Ocampo   +12 more
wiley   +1 more source

Design of Single‐Atom Catalysts Anchored in N‐Doped Biphenylene Using Symbolic Regression for Electrocatalytic Nitrate Reduction to Ammonia

Advanced Science, EarlyView.
A high‐throughput in silico calculations for NO3RR based on transition metal doped and nitrogen decorated biphenylene network are performed. A symbolic regression is designed to capture the hidden descriptors of NO3RR for hyper dimensional system entailing large geometric variability.
Zheng Shu, Zhangsheng Shi, Huaxian Jia, Huifang Xu, Zian Xu, Zhongheng Li, Man‐Fai Ng, Teck Leong Tan, Fuqiang Huang, Yongqing Cai   +9 more
wiley   +1 more source