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Key Drivers of Activity and Selectivity in Cu‐Based Catalysts for Methanol Synthesis From CO2: Insights From Atomically Dispersed Promoters

Angewandte Chemie, EarlyView.
Mechanistic studies on model Cu─M/SiO2 catalysts (M = Zn, Ga, and In) reveal that promoters enable a formate spillover pathway from Cu to Mn+ (n = 2 or 3) sites. The promoter's electronic effect on formate bond strengths serves as a quantitative descriptor for activity and selectivity, balancing spillover dynamics with intermediate stabilization to ...
Nat Phongprueksathat +6 more
wiley +1 more source

Adenylation Domain Engineering Enables Biosynthesis of an Improved Polymyxin Antibiotic

Angewandte Chemie, EarlyView.
To enable incorporation of l‐2‐aminodecanoic acid into polymyxin by fermentation, a single Trp‐to‐Ala substitution is rationally introduced into the adenylation‐domain residue of its nonribosomal peptide synthetase (NRPS) and efficiently switches substrate selectivity. The engineered strain produces biologically active Ada‐polymyxin, demonstrating that
Maximilian Müll +7 more
wiley +1 more source

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combates - rituais

Sérgio Buarque de Holanda em combates com Alceu Amoroso Lima: o tomismo na tópica do atraso

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Combates e continuidades do legado modernista em algumas publicações contemporâneas

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Os rituais de passagem segundo adolescentes

ACTA Paulista De Enfermagem, 2008
Thaïs Fernanda Vieira, Danila Cristina Paquier Sala +1 more
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Combates verbales en elCantar de Mio Cid

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Alfonso Boix Jovani
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Teatro do Oprimido e projeto emancipatório: mutações, fragilidades e combates

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Fernando Ilidio Ferreira
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