Results 161 to 170 of about 3,602,068 (194)

APTES‐Mediated Ti‐Squarate MOF/n‐GaN Nanowire Photoanodes for Efficient Photoelectrochemical Water Splitting

open access: yesAdvanced Functional Materials, EarlyView.
The APTES linker establishes a permanent interfacial dipole, reducing the work function of n‐GaN from 3.55 to 3.29 eV. This strengthens the built‐in electric field, significantly accelerating hole extraction to drive the oxygen evolution reaction (OER). Ultimately, this tailored charge‐separation architecture achieves a remarkable 4.78‐fold enhancement
Jeong‐Kyun Oh   +15 more
wiley   +1 more source

Bistable Isochoric Chiral Metamaterials with Reprogrammable Multiaxial Responses

open access: yesAdvanced Functional Materials, EarlyView.
An isochoric bistable rotational unit cell enables in situ modification of internal contact conditions post‐fabrication, without altering the global envelope dimensions of the surrounding architecture. By selectively switching between open and closed states, the tessellated chiral metamaterial can reprogram its volumetric response, including bulk ...
Shujia Chen   +3 more
wiley   +1 more source

In Situ Interfacial Assembly of Dynamic Semi‐Interpenetrating Biopolymer Networks for Robust and Mechanically Adaptive Droplet Interfaces

open access: yesAdvanced Functional Materials, EarlyView.
A dynamic interfacial semi‐interpenetrating polymer network is constructed by sequential assembly of β‐sheet‐rich SF and CS‐RL. The SF framework provides mechanical strength, while dynamically associated CS‐RL enables local rearrangement, allowing droplets to rapidly reconfigure without loss of interfacial integrity.
Yaping Zhang   +7 more
wiley   +1 more source

Tantalum–Palladium Ultrathin Resistance Hydrogen Sensor

open access: yesAdvanced Functional Materials, EarlyView.
Nanoconfined Ta‐alloy thin films enable fast, reversible hydrogen sensing by suppressing unwanted phase transitions. A Ta0.88${\rm Ta}_{0.88}$Pd0.12${\rm Pd}_{0.12}$ sensing layer delivers hysteresis‐free detection from ppb to 100% H2${\rm H}_2$ at room temperature.
Folkert Isaäc Bernhard Straus   +2 more
wiley   +1 more source

Endosomal Escape of siRNA Polyplexes: A Molecular Dynamics Perspective on Underlying Mechanisms

open access: yesAdvanced Functional Materials, EarlyView.
Molecular dynamics simulations reveal distinct endosomal escape mechanisms of siRNA nanoparticles, ranging from electrostatic membrane attachment to hydrophobic membrane fusion. Hydrophobic residues and anionic endosomal lipids emerge as key determinants of membrane disruption, linking molecular interactions to experimental delivery performance and ...
Katharina M. Steinegger   +5 more
wiley   +1 more source

Programming Neuromorphic Plasticity Through Ionic and Electronic Coupling in Organic Electrochemical Transistors

open access: yesAdvanced Functional Materials, EarlyView.
Neuromorphic plasticity in OECTs is governed by the post‐stimulus evolution of coupled ionic and electronic states. Semiconductor chemistry and morphology, electrolyte composition and interfaces, and device architecture regulate ion injection, transport, confinement, and release, shifting responses from rapidly relaxing STP to metastable memory and ...
Inho Lee   +9 more
wiley   +1 more source

Ultra‐Thin Tow‐Based Discontinuous Composites—Material Overview and Aspirations

open access: yesAdvanced Functional Materials, EarlyView.
Tow‐based discontinuous composites made from ultra‐thin tapes offer outstanding in‐plane mechanical properties. This material, inspired by Nacre, has high volume fraction of tapes exceeding 90 % and allows for quasi‐isotropic material plates less than 100 micrometer in thickness.
Ioannis Katsivalis   +8 more
wiley   +1 more source

Beyond Primary Nucleation: Molecular Basis of Peptide Crystal Secondary Nucleation at Soft Interface

open access: yesAdvanced Functional Materials, EarlyView.
High spatiotemporal‐resolution atomic force microscopy directly resolved peptide secondary nucleation (SN) and growth characteristics and mechanisms on HOPG. The landscape of peptide nucleation sites, growth dynamics, molecular‐scale structures, phase transitions, and cross‐seeding processes were realized.
Linhao Sun   +2 more
wiley   +1 more source

How the Porous Transport Layer Dictates Membrane Electrode Assembly Performance of IrO2 Catalysts

open access: yesAdvanced Functional Materials, EarlyView.
The Schottky barrier formed at the catalyst | PTL interface critically governs both the initial performance and long‐term durability of the PEMWE, and its magnitude is dictated by the catalyst's work function. This limitation can be resolved by combining a rutile IrO2 core for efficient electron transfer with an amorphous IrOx shell for high surface ...
Hyeseong Jeon   +6 more
wiley   +1 more source

Self‐Adaptive Gradient Interphase Enables Durable Solid‐State Lithium Metal Batteries

open access: yesAdvanced Functional Materials, EarlyView.
This work presents a machine learning‐guided interfacial design that forms a self‐adaptive graded interphase on lithium metal anode. A B105M40 composite interlayer evolves into lithiophilic, porous, and fast‐ion‐conducting phases, enabling intimate contact, dendrite suppression, and uniform lithium deposition.
Hongmin Liu   +9 more
wiley   +1 more source

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