Results 191 to 200 of about 39,200 (261)

A Perspective on the Origin of High‐Entropy Solid Electrolytes

open access: yesAdvanced Materials, EarlyView.
This perspective critically examines HE approaches in SEs, highlighting how compositional complexity induces system disorder and local‐structure evolution to enhance stability and properties. While HE concepts are attractive, establishing rigorous structure‐property relationships requires further investigation.
Feipeng Zhao, Shumin Zhang, Xueliang Sun
wiley   +1 more source

Harnessing Synergistic Cooperation of Neighboring Active Motifs in Heterogeneous Catalysts for Enhanced Catalytic Performance

open access: yesAdvanced Materials, EarlyView.
This review examines the critical role of neighboring active motifs in heterogeneous catalysts, emphasizing how their synergistic cooperativity can be rationally designed to modulate catalytic properties. The discussion centers on the modulation of electronic and geometric structures, categorizing the catalytic systems into metal‐acid (Brønsted/Lewis ...
Peng Yuan   +2 more
wiley   +1 more source

Efficient Low‐temperature Ammonia Cracking Enabled by Strained Heterostructure Interfaces on Ru‐free Catalyst

open access: yesAdvanced Materials, EarlyView.
Leveraging the strong metal‐support interaction effect, heterostructured interfaces in a Co‐based catalyst are designed to enable low‐temperature ammonia (NH3) decomposition. The induced tensile lattice strain within the core‐shell structure modulates d‐band center of Co, enhancing NH3 adsorption and facilitating N─H bond dissociation. Furthermore, the
Pei Xiong   +10 more
wiley   +1 more source

Toward Zero‐Excess Alkali Metal Batteries: Bridging Experimental and Computational Insights

open access: yesAdvanced Materials, EarlyView.
This review explores zero‐excess alkali metal batteries, highlighting anode–electrolyte interfaces, metal nucleation, dendrite growth, and SEI formation while comparing Li, Na, and K metals. It critically examines electrolyte and separator roles, emphasizing substrate design, electrolyte modifications, interfacial engineering, and solid‐state ...
Pan He   +6 more
wiley   +1 more source

Recent Advances in Heterogeneous Frustrated Lewis Pair: Synthesis, Characterization, and Catalysis

open access: yesAdvanced Materials, EarlyView.
This review provides a concise analysis of heterogeneous frustrated Lewis pair (FLP) chemistry, focusing on their synthesis, characterization, and application in small‐molecule activation. It highlights current challenges in developing solid FLP systems and explores promising advancements through emerging technologies, offering critical insights into ...
Jiasi Li   +2 more
wiley   +1 more source

Circuit complexity and functionality: A statistical thermodynamics perspective. [PDF]

open access: yesProc Natl Acad Sci U S A
Chamon C   +3 more
europepmc   +1 more source

Designing the Self‐Assembly of Disordered Materials Via Color Frustration

open access: yesAdvanced Materials, EarlyView.
What if disorder can be designed? This work introduces a strategy to self‐assemble amorphous materials by designing bonding rules for patchy particles that suppress crystallinity and promote frustration. The designer particles nucleate a network of dodecahedral cages from the liquid, yielding a novel equilibrium amorphous phase. This approach redefines
Andreas Neophytou   +2 more
wiley   +1 more source

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