Results 121 to 130 of about 2,646,324 (273)

Closed‐Loop Solid‐State Synthesis Planning for Materials Discovery With Large Language Models

open access: yesAdvanced Materials, EarlyView.
Leveraging literature data, we build a large‐language‐model‐driven workflow that extracts synthesis steps from 4407 papers, retrieves similar precedents, and generates candidate solid‐state synthesis recipes. The system benchmarks against ground‐truth and then operates in a closed loop with experiments to synthesize oxy‐selenide electrolyte materials ...
Dong Won Jeon   +9 more
wiley   +1 more source

Specific Position of Halogen in Crystalline TADF Scintillators Enables Efficient Triplet Harvesting Through Vibrational Modulation of Spin–Orbit Coupling

open access: yesAdvanced Materials, EarlyView.
Specific ortho‐halogenation transforms crystalline TADF emitters into efficient organic scintillators. Fluorine reduces the effective singlet–triplet separation, while chlorine combines near‐degenerate excited states with vibrational modulation of spin–orbit coupling.
Illia E. Serdiuk   +8 more
wiley   +1 more source

Stress Transfer Within Microphase‐Separated Structures: A Post‐Synthetic Strategy to Impart Mechanoresponsiveness to Block Copolymer Materials

open access: yesAdvanced Materials, EarlyView.
A domain‐engineered post‐functionalization strategy is presented to impart mechanochromism to styrene–butadiene–styrene (SBS) block copolymers by simple blending with a tetraarylsuccinonitrile (TASN) mechanophore‐containing polystyrene (PS‐TASN‐PS). The resulting materials exhibit reversible fluorescence under tensile deformation while preserving, or ...
Kuniaki Ishizuki   +3 more
wiley   +1 more source

Defect‐Templated Phase Engineering in Atomically Thin Metals

open access: yesAdvanced Materials, EarlyView.
Graphene defects are transformed from passive imperfections into programmable templates for phase‐selective growth of atomically thin silver. Plasma‐generated boundary defects favor Ag(1), whereas sp3‐rich zero‐layer graphene promotes Ag(2). This defect‐directed intercalation links local graphene chemistry to crystalline phase, electronic structure ...
Arpit Jain   +25 more
wiley   +1 more source

Gamma-ray spectrometry

open access: yes, 2008
K Ford   +4 more
openaire   +1 more source

Side‐Chain‐Induced Interlayer Slipping in Metalloporphyrin COFs Enables Microenvironment and Spin‐State Regulation for Photocatalytic CO2 Reduction

open access: yesAdvanced Materials, EarlyView.
Alkoxy chain length drives a continuous transition from eclipsed AA to a serrated, slipped AA* configuration over Co‐porphyrin COFs. A moderate slip both contracts the pore channel to enrich CO2 and suppress hydrogen evolution, and enhances collective high‐spin of Co sites, which delivers a record CO production rate with high selectivity.
Jie He   +8 more
wiley   +1 more source

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