Results 141 to 150 of about 691,269 (288)

Operator-level quantum acceleration of non-logconcave sampling. [PDF]

Proc Natl Acad Sci U S A
Leng J, Ding Z, Chen Z, Lin L.
europepmc   +1 more source

Highly Efficient Extraction of 212 Pb/212Bi from the Decay Chain of 232Th‐Based on Anion Exchange in Bromide Medium

Advanced Science, EarlyView.
This work provides an effective strategy for selectively extracting 212Pb and 212Bi from the decay chain of 232Th as well as its mechanism illustration. Using the novel strategy, 2.07 MBq of 212Pb is successfully separated from 232Th and its daughters, which enables the supply of 212Pb/212Bi directly from the abundant natural thorium resource to be ...
Lifeng Chen, Wannian Feng, Yuezhou Wei, Xuexiang He, Shaoying Wang, Zhongyuan Zhou, Qiang Wu, Ningchao Zheng, Xiangbiao Yin, Wenlong Li, Lingling Su, Shunyan Ning   +11 more
wiley   +1 more source

Electride‐Induced Electronic Modulation of Ruthenium Catalyst for Highly Efficient Alkaline Hydrogen Evolution

Advanced Science, EarlyView.
Electrides offer unique opportunities as catalyst supports for hydrogen evolution reactions. This study presents an electride‐supported Ru/Nd2ScSi2 catalyst exhibiting outstanding hydrogen evolution reaction performance and excellent stability. Anionic Ru species on the electride surface facilitate water dissociation and optimize hydrogen adsorption ...
Zhiqi Wang, Jianan Su, Cheng Li, Yutong Gong, Hideo Hosono, Junjie Wang   +5 more
wiley   +1 more source

A Wood Plasticine With Controlled Phase‐Change Behavior and Malleability for Energy‐Closed‐Loop and Conformally Adaptive Thermal Management

Advanced Science, EarlyView.
A photothermal wood plasticine exhibiting controlled phase‐change behavior and malleable property is developed. The developed wood plasticine can provide all‐day, on‐demand, and low‐loss solar heating for geometrically diverse objects, including thermoelectric generator, human body, and battery, through its controlled crystallization‐melting ...
Jiazuo Zhou, Yifan Liu, Lei Qiao, Yuehe Gu, Taikun Yao, Wenbo Zhang, Fangmiao Wang, Yudong Li, Xinyao Ji, Lingyi Kong, Haiyue Yang, Yao Xiao, Chengyu Wang   +12 more
wiley   +1 more source

Redox‐Active Tungsten Mono‐Oxo Bis(dithiolene) Complex: A Fast‐Rechargeable Anode for High‐Capacity Lithium‐Ion Batteries

Advanced Science, EarlyView.
This study reports the first application of a W‐oxo bis(dithiolene) complex, (Et4N)2[WO(S2C2(C6H5)2)2], as a novel anode material for lithium‐ion batteries. This complex stores Li+ ions via multivalent W‐centered redox processes involving its oxo (WO) and dithiolene (S) sites.
Honggyu Seong, Jaeheon Lee, Jae Hyun Park, Woonghee Lee, Junhyeok Seo, Jaewon Choi   +5 more
wiley   +1 more source

Thermodynamically consistent machine learning model for excess Gibbs energy. [PDF]

Nat Commun
Hoffmann M, Specht T, Göttl Q, Burger J, Mandt S, Hasse H, Jirasek F.   +6 more
europepmc   +1 more source

Heterointerface‑Enabled Electrocatalysis for Efficient Energy Conversion

Advanced Science, EarlyView.
Functionally distinct A/B materials can be integrated at the nanoscale to create customized heterointerfaces with tunable band alignment and charge redistribution, providing fast electron and ion transport channels as well as cooperative dual active sites.
Liuru Fang, Hsiwen Wu, Hengyue Xu, Jie Zhang   +3 more
wiley   +1 more source

Atomistic Model for Water Adsorption in Mg-MOF-74: Quantum Chemical Prediction of Structures and Isotherms. [PDF]

J Am Chem Soc
Mancini N, Berger F, Rybicki M, Sillar K, Sauer J.   +4 more
europepmc   +1 more source

Epitaxial Stabilization of Ultrasmall Cu Nanoparticles With High‐Energy {110} Facets on Ti3C2 MXene for Efficient CO2‐to‐Acetate Electrocatalysis

Advanced Science, EarlyView.
Cu/Ti3C2 heterostructure: Cu/Ti3C2 heterostructure achieves epitaxial stabilization of high‐energy Cu(110) facets through lattice matching and electronic interaction, enabling efficient CO2 electroreduction to acetate with 42.5% Faradaic efficiency at 235 mA·cm−2. ABSTRACT The electrochemical CO2 reduction reaction (CO2RR) to multicarbon (C2+) products
Yan‐An Li, Jiapeng Huang, Yaohui Zhao, Junhao Lu, Yuan Ren, Zi‐Xin Ge, Qian Wang, Shangdong Ji, Yangzi Zheng, Chao Wu, Mingshang Jin   +10 more
wiley   +1 more source

Substrate‐Affinitive P‐Type Azapolycyclic Photosensitizer for Chemoselective Nitrilization Under Mild Conditions

Advanced Science, EarlyView.
We developed a series of quinoxalinoquinoxaline (QQ) photosensitizers featuring high and tunable excited‐state reduction potentials (E(PC•+/PC*) = –1.76 to –2.05 V vs. SCE). Their hydrogen‐bonding interaction with carbonyl substrates enables selective single‐electron transfer events for selective nitrilization of 1° amides, offering a tunable ...
Seongwoo Bae, Dongwook Kim, Jinwoo Kim
wiley   +1 more source