Results 181 to 190 of about 183,644 (280)

Mitigating the Rock‐Salt Phase Transformation in Disordered LNMO Through Synergetic Solid‐State AlF3/LiF Modifications

Advanced Science, EarlyView.
The transition between the spinel and rock‐salt phases induces irreversible structural changes in disordered LiNi0.5Mn1.5O4, thereby preventing it from fully releasing its electrochemical capacity during charge/discharge cycling. Abstract High‐voltage disordered spinel LiNi0.5Mn1.5O4 is a promising cathode material for high power density in lithium‐ion
Xingqi Chang, Carlos Escudero, Ashley P Black, Sharona Horta, Elías Martínez, Xuan Lu, Jordi Llorca, Maria Ibáñez, Jordi Jacas Biendicho, Andreu Cabot   +9 more
wiley   +1 more source

Valence‐Engineering of CeO2 Redox Modulator Boosts the Oxygen Electrocatalysis Performance in Fe/Co Dual‐Atom Catalyst

Advanced Science, EarlyView.
Valence‐engineering of CeO2 redox modulator can remove the highly oxidative by‐products and accelerate the oxidation state transitions of Co/Fe centers in FeCo dual‐atom catalyst during oxygen reduction/evolution electrocatalysis. Therefore, the stability and activity issues are resolved, significantly enhancing the overall performance when used as an ...
Hengqi Liu, Jinzhen Huang, Shengyu Ma, Rui Xiong, Jiong Zhao, Qiang Fu, Hang Wei, Zhiguo Liu, Xianjie Wang, Tai Yao, Bo Song   +10 more
wiley   +1 more source

Iron/Cobalt Dual‐Atom Catalyst Orchestrate Photothermal‐Chemodynamic Immunotherapy Against MRSA: Multi‐Omics Dissection in Murine and Porcine Models

Advanced Science, EarlyView.
FeCo dual‐atom catalyst (FeCo‐N‐DAC) with ultrahigh metal loading (Fe > 5.4%, Co > 4.8%) is developed for synergistic photothermal‐chemodynamic immunotherapy. FeCo‐N‐DAC penetrates deep‐seated tissues, eradicates MRSA biofilms, and reprograms immune‐inflammatory pathways via multi‐omics‐validated mechanisms.
Shihao Xu, Binge Huang, Hao Lin, Jinming Li, Zhaoxiang Lu, Qi Zhang, Jia Li, Shiping Yang, Songsong Lan, Yan Yang, Yun Feng, Xiaojun He   +11 more
wiley   +1 more source

Islet Amyloid Polypeptide Modelled to Simulate Diabetes Co‐Oligomerized with β‐Amyloid 1‐42 Reproducing the Pathological Cascade of Alzheimer's Disease in Human Cerebral Organoids

Advanced Science, EarlyView.
Human islet amyloid polypeptide (hIAPP) was used to mimic T2DM, and Aβ42‐hIAPP co‐oligomers were delivered into the human mature cerebral organoids (COs), which reproduce typical AD pathology and significant neuronal death more closely resembling that of AD patients.
Jin Yan, Zhimeng Tang, Yanyu Luo, Bin Liu, Xinxin Huang, Jun Wei, Feng Yue   +6 more
wiley   +1 more source

Superelastic High‐Entropy Oxide Ceramic Aerogels for Thermal Superinsulation and Sealing at Extreme Conditions

Advanced Science, EarlyView.
A high‐entropy oxide ceramic of (Gd1/2Lu1/2)2(Ti1/3Zr1/3Hf1/3)2O7 is prepared through a molecular synthesis route of pyrolytic solid‐solution reactions. The architectured nanofiber aerogel manifests unprecedented thermomechanical properties, including superelastic compressibility of 98% from −196 to 1500 °C, and thermal superinsulation capacity (24.14 ...
Xiaoke Jiang, Tao Du, Hengzhong Fan, Junhong Liu, Yunfeng Su, Peng He, Hongxiang Chen, Litian Hu, Yongsheng Zhang, Qiangqiang Zhang   +9 more
wiley   +1 more source

Asymmetric Active Center Triggers Side‐On Photo‐Fenton‐Like Reaction Through Polar Charge Transfer and Self‐Adapting Sulfur Vacancies

Advanced Science, EarlyView.
The Cu‐Zn3In2S6 photocatalyst (Cu‐ZISV) with asymmetric Cu‐SV‐Zn sites was designed and synthesized to boost peroxymonosulfate (PMS) activation kinetics. The side‐on photo‐Fenton‐like reaction by the asymmetric Cu‐SV‐Zn site accelerated PMS activation and pollutant degradation, and the first‐order kinetic constant of Cu‐ZISV increased by 4.87 times ...
Jiaqi Hu, Xiaoyuan Zhang, Yufei Gao, Jianyi Liu, Xu He, Yu Liu, Jinfeng Lu, Jun Ma   +7 more
wiley   +1 more source

In Situ Construction of Cu1+/Cu0 and Cu2+/Cu0 Pairs of Cu‐Based Catalysts for Electrocatalytic Nitrate Reduction

Advanced Science, EarlyView.
CuO and CuPO (Cu2P2O7 and Cu3(PO4)2) as precursors are in suit construction two distinct copper‐based active sites during the NO3RR reaction: Cu1+/Cu0 (derived from CuO) and Cu2+/Cu0 (derived from CuPO). Cu1+/Cu0 is the key to achieving high activity and high selectivity.
Shanna An, Jiali Ren, Yanjun Xue, Jian Tian   +3 more
wiley   +1 more source

Unraveling the Origin of Exceptional Activity in NiMo Alloys for Alkaline Hydrogen Evolution

Advanced Science, EarlyView.
This study resolves the controversy regarding the active origin of Nickel‐molybdenum (NiMo) alloys for alkaline hydrogen evolution. By combining surface Pourbaix diagrams with microkinetic modeling, we demonstrate that the O‐covered Ni3Mo surface drives activity through a synergistic mechanism: Mo sites facilitate water dissociation while adjacent Ni ...
Yuefeng Zhang, Wenqiang Yang, Zhiyuan Zeng, Zhen‐Yu Wu, Zhenbin Wang   +4 more
wiley   +1 more source

Enhanced Oxygen Redox Activity and Structure Stability of P2‐Type Manganese‐Based Cathodes Through Medium‐Entropy Strategy

Advanced Science, EarlyView.
A medium‐entropy strategy guided by ionic potential is applied to weaken TM─O bonds and suppress Jahn–Teller distortion in P2‐type cathodes, thereby enhancing the oxygen redox activity and structure stability. A medium‐entropy oxide, Na0.8Li0.1Ni0.1Cu0.1Ti0.1Mn0.6O2, demonstrates a high reversible capacity of 223.7 mAh g−1 and an energy density of 616 ...
Dongxiao Wang, Yuxuan Liu, Zihao Wang, Wei Su, Xingguo Qi, Huican Mao, Kan Zhang, Shigang Lu, Bingkun Guo, Yingchun Lyu   +9 more
wiley   +1 more source

Room‐Temperature Alane Dehydrogenation for Visible‐Light‐Driven Photocatalytic Hydrogen Supply System

Advanced Science, EarlyView.
In situ formed Al/MOF enables viable visible‐light‐driven photocatalytic dehydrogenation of alane (AlH3) confirming practical application. Results demonstrate that Al nanoparticles prolong lifetime of photogenerated charge carriers via localized surface plasmon resonance induced hot electron injection, while AlH3 chemisorption triggers interfacial ...
Ting‐Ting Li, Li‐Cheng Liang, Rui‐Qi Chen, Chun‐Qi Zhang, Sheng‐Nan Zhang, Wen‐Wen Cheng, Xi‐Hao Chen, Ning Wang, Juan‐Ding Xiao, Qing‐Qing Yang, Fei Liang, Chao‐Feng Zhang   +11 more
wiley   +1 more source