Results 171 to 180 of about 12,927,323 (257)

Decoupling Stable Cyclic Deformation From Defect Accumulation in Metals

Advanced Science, EarlyView.
Introducing amorphous nanoparticles into a metal matrix enables a cyclic deformation regime where strain hardening and defect accumulation are decoupled. These nanoparticles act as dislocation sinks and undergo reversible shear transformations, sustaining microstructural stability over millions of cycles.
Chenjun Ye, Shaofan Ge, Tian Yang, Leyi Tang, Kang Wang, Y. Morris Wang, Jun Ding, Zan Li, Di Zhang, En (Evan) Ma   +9 more
wiley   +1 more source

Deciphering Electrochemical Generation, Transport, and Reactivity of Hydrogen Species in the Electrochemical Palladium Membrane Reactor

Advanced Science, EarlyView.
This study elucidates hydrogen transport and reaction mechanisms in ePMR using 1‐hexyne hydrogenation as a model reaction. Hydrogen transport operates via dual pathways involving hydrogen atom permeation and H2‐mediated re‐dissociation on secondary metal layers.
Samuel J. Shin, Su Bin Roh, Hyun‐Tak Kim, Kwan‐Young Lee, Soo Min Kim, Ji Hoon Park, Minju Park   +6 more
wiley   +1 more source

Thermally Regulated Methanol Selectivity in Photo‐Thermo Methane Oxidation Through Interfacial Methyl Transfer

Advanced Science, EarlyView.
Photo‐thermo cascade catalysis enables highly selective methane‐to‐methanol conversion over Au‐ZnO, achieving a CH3OH production rate of ∼800 µmol h−1 with 86% selectivity. Thermal activation gates the transfer of methane‐derived methyl intermediates from ZnO to Au, thereby redirecting the reaction pathway toward methanol formation. ABSTRACT The direct
Youxun Xu, Chengzhi Guo, Chaoran Jiang, Leirun Chen, Juncong Wang, Enqi Chen, Yang Lan   +6 more
wiley   +1 more source

The Potential of Zero Charge: An Interfacial Descriptor Governing Hydrogen Evolution Reaction on Bulk Metal Electrodes

Advanced Science, EarlyView.
This work establishes a dual‐descriptor framework incorporating hydrogen adsorption free energy and potential of zero charge, constructing a corrected 3D HER volcano plot. It reveals that surface charge and interfacial proton concentration jointly govern activity, beyond conventional 2D thermodynamic scaling relations. ABSTRACT While the Sabatier‐based
Yuefei Zhang, Yufei Xue, Yang Zhang, Xuefei Liu, Aijun Du, Lin‐wang Wang, Guoping Gao   +6 more
wiley   +1 more source

Mental Health Reform [PDF]

North Carolina Medical Journal, 2004
openaire   +2 more sources

Intelligent Polymer Electrolytes for Next‐Generation Zinc‐Based Energy Storage Devices

Advanced Science, EarlyView.
Intelligent polymer electrolytes are organized into a three‐level hierarchy that advances zinc‐based energy storage from passive ion conduction toward active, adaptive, and intelligent operation. Molecular regulation of Zn+ coordination, water activity, desolvation, ion flux, and interfaces underpins adaptive self‐healing, anti‐freezing, adhesion, and ...
Sanath Kumar, Jhansirani Kesavan, Muhammad Asim, Atul Verma, Yen‐Pei Fu   +4 more
wiley   +1 more source

Electrocatalytic Urea Synthesis From CO2 and N2/NO3−: Bridging Catalyst Activity, C–N Coupling Kinetics, and Industrial Applicability

Advanced Science, EarlyView.
This review compares NO3− + CO2 and N2 + CO2 electrocatalytic urea synthesis in feedstock properties, catalyst design, C–N coupling mechanisms, performance optimization, and engineering applicability. The two systems correspond to a near‐term deployable route and a long‐term green synthesis goal, respectively.
Fulin Dong, Ruihan Zhang, Huiyu Lou, Tianshi Gao, Guangjin Zhang, Menglei Yuan   +5 more
wiley   +1 more source

Glycerol‐Regulated Cytocompatible, Self‐Healing Gel Electrolyte Stabilizes Zinc Metal Anodes for Quasi‐Solid‐State Aqueous Batteries

Advanced Science, EarlyView.
A glycerol‐regulated PVA/PEG self‐healing gel electrolyte reconstructs the hydrogen‐bonding and Zn2+ coordination environments, suppressing water‐related parasitic reactions and enabling regulated Zn nucleation and homogeneous deposition. The resulting quasi‐solid‐state electrolyte combines durable Zn‐metal reversibility, self‐healing functionality ...
Yuchuan Ren, Qian Xue, Lihong He, Canhuang Li, Ruixia Li, Xiaoyu Bi, Jiali Chai, Yapeng Cheng, Tiezhu Guo, Andreu Cabot   +9 more
wiley   +1 more source

Weak‑Solvation‑Mediated Localized High‑Concentration Electrolyte for Sodium Metal Batteries

Advanced Science, EarlyView.
A weak‑solvation strategy using MTBE as a fluorine‑free diluent constructs a localized high‑concentration structure, promoting FSI− coordination and forming an inorganic‑rich SEI. This enables stable cycling with high‑loading cathodes and pouch cells, offering a sustainable, PFAS‑free electrolyte for sodium metal batteries.
Hongxu Qu, Huihua Li, Jingxuan Wang, Mingxing Zhang, Yang Wang, Yuhang Meng, Sailei Shao, Stefano Passerini, Huang Zhang   +8 more
wiley   +1 more source

From Materials to Systems: Challenges and Solutions for Fast‐Charge/Discharge Na‐Ion Batteries

Advanced Energy Materials, EarlyView.
This review systematically analyzes the key characteristics limiting the fast‐charge/discharge capability of Na‐ion batteries (SIBs) from a multi‐scale perspective encompassing electrode materials, the electrode‐electrolyte interface, and the system. Furthermore, it presents practical solution strategies for the fundamental issues arising at each scale,
Bonyoung Ku, Sangbin Park, Sunha Hwang, Sunghyun Lim, Won‐Sub Yoon, Jongsoon Kim   +5 more
wiley   +1 more source