Enhancing Triplet Excitons Lifetime Through Controlled Intermolecular Interactions
Advanced Optical Materials, EarlyView.Singlet fission (SF) is investigated in pentacene embedded in a surface‐anchored metal–organic framework, enabling a molecular arrangement inaccessible in pure organic crystals. This architecture changes the singlet fission dynamics significantly and enhances the triplet lifetime by almost four orders of magnitude.
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