Results 101 to 110 of about 48,082 (256)

Unifying Composition and Process Design: A Heterogeneous Graph Neural Network for Discovering High‐Performance Cu Alloys

open access: yesAdvanced Science, EarlyView.
By overcoming the fixed‐path limitations of conventional machine learning, a heterogeneous graph neural network fundamentally reconstructs material data representation. Integrating variable processing sequences with intrinsic elemental features, this framework enables exploratory optimization across high‐dimensional spaces.
Jie Yin   +12 more
wiley   +1 more source

Comparative analysis of inductively coupled plasma mass spectrometry and alpha spectrometry methods to measure plutonium activity in biosubstrates

open access: yesРадиационная гигиена
Currently, the most common methods to measure the activity of transuranium elements in biological samples are alpha radiometry and alpha spectrometry. Of these, alpha spectrometry is the most sensitive and selective method.
V. R. Batalov   +3 more
doaj   +1 more source

Operando Electrochemical Formation of Integrated Ni‐Fe Oxyhydroxide Anode for Durable Anion Exchange Membrane Water Electrolyzer

open access: yesAdvanced Science, EarlyView.
The interfacial stability and activity of Ni‐Fe‐based AEMWE anodes can be directly enhanced by operando voltage‐cycling in a FeOOH‐containing electrolyte. This process simultaneously induces Ni oxidation and Fe incorporation, forming an integrated, porous (Fe, Ni)OOH layer with high conductivity and durability.
Euntaek Oh   +10 more
wiley   +1 more source

Efficient Direct Recycling of Spent Batteries: Integrated Lithiation and Delamination

open access: yesAdvanced Science, EarlyView.
An integrated process for the delamination and relithiation of spent cathodes, LixNi0.6Co0.2Mn0.2O2 and LixFePO4, under open‐air conditions is proposed. The transition‐metal (Ni) oxidation state in the cathode is reduced by the oxidation of diethylene glycol, facilitating relithiation. Glycol aldehyde formation induces 100% electrode delamination.
Jeonghwan Song   +11 more
wiley   +1 more source

Near‐Unity Selectivity Inversion Between CO2 Electroreduction and H2 Evolution via Atomic Coordination Editing

open access: yesAdvanced Science, EarlyView.
Atomic coordination editing functions as an on/off switch that toggles single‐atom catalysts between CO2 electroreduction and hydrogen evolution. ABSTRACT Precise atomic coordination editing of single‐atom catalysts (SACs) provides an effective strategy to tune their electronic structures and catalytic selectivity. Yet, achieving near‐unity selectivity
Yukun Zhao   +11 more
wiley   +1 more source

Al─N Co‐Doped LLZO Solid Electrolytes via One‐Step Sintering: Toward High Ionic Conductivity

open access: yesAdvanced Science, EarlyView.
Al–N co‐doped LLZO solid electrolytes were prepared via a one‐step sintering process, which not only simplifies fabrication process, but also diminishes Li loss during high‐temperature sintering in conventional fabrication process. The Al–N co‐doped LLZO achieves a high ionic conductivity of 2.19 × 10−3 S cm−1 because the co‐doping reduces the energy ...
Hao Zhang   +9 more
wiley   +1 more source

Machine Learning‐Assisted KCl‐CaCl2‐LiCl Electrolyte Design for Low‐Temperature, High‐Performance Calcium‐Based Liquid Metal Batteries

open access: yesAdvanced Science, EarlyView.
A machine learning‐assisted framework optimizes the KCl‐CaCl2‐LiCl ternary electrolyte. The optimized 13:35:52 mol% composition enables Ca‐based liquid metal batteries to operate stably at 480 °C, with >99.5% coulombic efficiency, ultralow self‐discharge, and excellent cycling stability, advancing low‐temperature large‐scale energy storage.
Xinglin Zhou   +3 more
wiley   +1 more source

Interfacial Proton‐Relay Microenvironment Enables Self‐Driven Singlet Oxygen Generation under Neutral Conditions

open access: yesAdvanced Science, EarlyView.
An interfacial proton‐relay microenvironment at MoS2‐CuCl heterostructures enables selective O2 activation to 1O2 under neutral conditions. Electron‐deficient sulfur sites mediate proton transfer to Cu‐bound O2, accelerating *OOH hydrogenation while suppressing O─O bond cleavage, achieving stable, efficient pollutant removal.
Qiaoyu Gao   +9 more
wiley   +1 more source

Dynamic Reconstruction‐Engineered Heterointerfaces for Acidic Hydrogen Evolution at Ampere‐Level Current Density

open access: yesAdvanced Science, EarlyView.
A dynamic reconstruction strategy was utilized to construct PtCu/Cu3P heterostructures on the surface of self‐supporting Cu3P nanowires. The loose porosity in the restructured layer, together with a dynamic “dissolution‐redeposition” equilibrium during electrocatalysis, enables the electrode to maintain a low, stable overpotential for 240 h at ampere ...
Kaixi Wang   +3 more
wiley   +1 more source

A High‐Current‐Tolerant Multimetallic Phosphide Electrode for Alkaline Water Electrolysis Toward Industrial Conditions

open access: yesAdvanced Science, EarlyView.
A phosphide‐modified multimetallic HER electrode achieves industrial‐level performance with minimal noble‐metal content. It delivers 1.7 A cm−2 at 2.0 V in 6 M KOH at 70°C and operates stably for over 200 h at 500 mA cm−2. Phosphorus tuning of the electronic structure optimizes hydrogen adsorption, offering a durable, high‐rate pathway for alkaline ...
Yang Li   +5 more
wiley   +1 more source

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