Results 111 to 120 of about 529,483 (274)

Methylation‐Induced Permanent Charge Polarization in Covalent Organic Frameworks for Visible Light‐Driven Water Decontamination and Disinfection

open access: yesAdvanced Science, EarlyView.
A targeted in situ methylation strategy is developed to engineer cationic centers in a quinoline‐linked COF (NQ‐COFS1‐Me), creating a strong built‐in electric field, which effectively suppresses excitonic effects and promotes charge separation. The optimized material demonstrates powerful photocatalytic ROS generation for rapid bacterial inactivation ...
Xuewen Peng   +7 more
wiley   +1 more source

T Cell Exhaustion in Cancer Immunotherapy: Heterogeneity, Mechanisms, and Therapeutic Opportunities

open access: yesAdvanced Science, EarlyView.
T cell exhaustion limits immunotherapy efficacy. This article delineates its progression from stem‐like to terminally exhausted states, governed by persistent antigen, transcription factors, epigenetics, and metabolism. It maps the exhaustion landscape in the TME and proposes integrated reversal strategies, providing a translational roadmap to overcome
Yang Yu   +7 more
wiley   +1 more source

Interfacially Coupled and Synergistic Effect of Ag/Co3O4‐C Nanocomposites for Enhanced Oxygen Reduction (ORR) and Evolution (OER) Reaction

open access: yesAdvanced Science, EarlyView.
Ag/Co3O4–C nanocomposites display well‐resolved lattice fringes and synergistic Ag/Co3O4 heterointerfaces that enhance charge transfer and active‐site exposure. The structural design enables superior bifunctional ORR/OER performance in alkaline media by promoting efficient adsorption and turnover of oxygen intermediates within an optimized ...
Adnan Qaseem   +8 more
wiley   +1 more source

Electronic Modulation of K⁺‐Intercalated Polymeric Carbon Nitride via ─C≡N/─OH Functionalization for Efficient Photocatalytic H2O2 Production

open access: yesAdvanced Science, EarlyView.
K+ is successfully embedded in the PCN interlayers via a high‐temperature polymerization. The incorporation of K+ perturbs the local electronic structure via interaction with nitrogen lone pairs, narrowing the PCN bandgap, which exhibits superior photocatalytic performance, achieving a high H2O2 generation rate both in situ and under sunlight ...
Qingquan Xue   +8 more
wiley   +1 more source

Atomic Defects in Layered Transition Metal Dichalcogenides for Sustainable Energy Storage and the Intelligent Trends in Data Analytics

open access: yesAdvanced Science, EarlyView.
This review comprehensively summarizes the atomic defects in TMDs for their applications in sustainable energy storage devices, along with the latest progress in ML methodologies for high‐throughput TEM data analysis, offering insights on how ML‐empowered microscopy facilitates bridging structure–property correlation and inspires knowledge for precise ...
Zheng Luo   +6 more
wiley   +1 more source

Single‐Cell Dissection of Tumor‐Infiltrating Lymphocytes Reveals Cellular Architecture Predictive of Therapeutic Efficacy in Acral Melanoma

open access: yesAdvanced Science, EarlyView.
Autologous tumor‐infiltrating lymphocyte (TIL) therapy shows promising efficacy in acral melanoma, yet determinants of durable response remain unclear. By integrating single‐cell transcriptomics and TCR sequencing, this study reveals that TIL products enriched for T follicular helper and intermediate exhausted T cells establish persistent clonal ...
Chao Zhang   +12 more
wiley   +1 more source

Non‐Equilibrium Synthesis Methods to Create Metastable and High‐Entropy Nanomaterials

open access: yesAdvanced Science, EarlyView.
ABSTRACT Stabilizing multiple elements within a single phase enables the creation of advanced materials with exceptional properties arising from their complex composition. However, under equilibrium conditions, the Hume–Rothery rules impose strict limitations on solid‐state miscibility, restricting combinations of elements with mismatched crystal ...
Shuo Liu   +3 more
wiley   +1 more source

Modulation of Electronic Structure in Kraft Lignin‐Derived Mo Single‐Atom Catalysts for Optimized Electrochemical Oxygen Reduction

open access: yesAdvanced Science, EarlyView.
Biomass‐derived lignin is used as a sustainable precursor to synthesize Mo single atoms anchored on a nitrogen‐coordinated carbon framework. As the Mo structure transitions from MoC clusters to isolated single‐atom sites, oxygen evolution reaction (ORR) activity progressively improves.
Junbeom Park   +16 more
wiley   +1 more source

Higher Education in Further Education and its impact on social mobility in England [PDF]

open access: yes
Further Education (FE) institutions in England have been providing a variety of higher education (HE) courses for decades. Despite the more recent expansion of HE in England, however, the proportion of those studying HE in FE colleges has remained ...
Orr, Kevin
core  

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