Results 141 to 150 of about 33,388 (259)

Stabilizing Cationic Palladium Single‐Atom Sites on Heteroatom‐Doped Carbon for Selective Hydrogen Peroxide Electrosynthesis

Advanced Functional Materials, EarlyView.
In this research, it is demonstrated that dual nitrogen and sulfur doping in hollow carbon spheres creates a tunable coordination environment that stabilizes cationic Pd single atoms as robust organometallic complexes, enabling high selectivity and stability for electrochemical hydrogen peroxide production under harsh acidic and peroxide‐rich ...
Guilherme V. Fortunato, Alexander Gunnarson, Hannaneh Hosseini, Xiangyu You, Pallabi Bhuyan, Ji Sik Choi, Hyo Sang Jeon, Xingshen Zhao, Julio C. Lourenço, Sumin Lim, Huize Wang, Ana Guilherme Buzanich, Martin Radtke, Paul Paciok, Marcos R.V. Lanza, Ferdi Schüth, Marc Ledendecker   +16 more
wiley   +1 more source

Charge‐Induced Morphing Gels for Bioinspired Actuation

Advanced Functional Materials, EarlyView.
This study introduces a novel electroactive actuation mechanism that enables the gel material to generate substantial and reversible shape‐changing while preserving topological and isochoric (volumetric) equivalence. The resultant morphing behaviors can mimic the movements of muscle‐driven organelles in nature, including cilia‐like beating and ...
Ciqun Xu, Saba Firouznia, Charl F. J. Faul, Majid Taghavi, Jonathan Rossiter   +4 more
wiley   +1 more source

Certified PEFTSmoothing: Parameter-Efficient Fine-Tuning with Randomized Smoothing

Randomized smoothing is the primary certified robustness method for accessing the robustness of deep learning models to adversarial perturbations in the l2-norm, by adding isotropic Gaussian noise to the input image and returning the majority votes over the base classifier.
Fu, Chengyan, Wang, Wenjie
openaire   +2 more sources

The Dynamics of Interfacial Trap States in High‐Detectivity Near‐Infrared Photomultiplication Organic Photodetectors

Advanced Functional Materials, EarlyView.
Photomultiplication organic photodetectors (PM OPDs) are an attractive strategy for health‐monitoring. Here, PM‐OPDs are reported with a specific detectivity of 5.7 × 1012 Jones and external quantum efficiency values of 3500% under −10 V. The dynamics of carrier trapping in these devices are elucidated through trap selective spectroscopical techniques.
Marie Houot, Zhuoran Qiao, Beier Hu, Davide Nodari, Francesco Furlan, Filip Aniés, Yicheng Yang, Martin Heeney, Artem A. Bakulin, Nicola Gasparini   +9 more
wiley   +1 more source

XuanHuGPT: parameter-efficient fine-tuning of large language model in the field of traditional Chinese medicine. [PDF]

Chin Med
Tong X, Ding X, Jia H, Yuan Y, Liu L, Wang Y, Xiong Z, Yang X, Im SK, Wang MH.   +9 more
europepmc   +1 more source

Multiple Twinning in Nacre and Aragonite

Advanced Functional Materials, EarlyView.
Electron backscatter diffraction map of a cluster of geologic aragonite, exhibiting single, double, and triple twins. The whole cluster is approximately 2 cm wide. Colors indicate crystal orientations, so that pixels where the a‐, b‐, and c‐axis is perpendicular to the image plane are green, red, and blue, respectively.
Connor A. Schmidt, William O. Nachlas, Bil Schneider, Xiaoming Mao, Eric Tambutté, Alexander A. Venn, Sylvie Tambutté, Pupa U. P. A. Gilbert   +7 more
wiley   +1 more source

Solvent‐Free Bonding Mechanisms and Microstructure Engineering in Dry Electrode Technology for Lithium‐Ion Batteries

Advanced Functional Materials, EarlyView.
Dry electrode technology revolutionizes battery manufacturing by eliminating toxic solvents and energy‐intensive drying. This work details two promising techniques: dry spray deposition and polymer fibrillation. How their unique solvent‐free bonding mechanisms create uniform microstructures for thicker, denser electrodes, boosting energy density and ...
Yuhao Liang, Hao Long, Zimo Huang, Ting He, Xueming Chen, Meng Li, Hao Chen, Shanqing Zhang   +7 more
wiley   +1 more source

High-fidelity parameter-efficient fine-tuning for joint recognition and linking of diagnoses to ICD-10 in non-standard primary care notes. [PDF]

JAMIA Open
Estupiñán-Ojeda C, Sandomingo-Freire RJ, Padró L, Turmo J.   +3 more
europepmc   +1 more source

Laser‐Based Sculpturing of Embedded Ultrathin Metal‐Oxide Nanopores for Enhanced Biomolecular Sensing

Advanced Functional Materials, EarlyView.
Controlled laser‐drilling of embedded HfO2 membranes creates three layer nanopores with Gaussian‐shaped cavities sculptured in the supporting layers. These embedded solid‐state nanopores slow DNA translocation by 12‐fold compared to SiNx pores, enabling high‐resolution, label‐free detection of short DNAs, RNAs, and proteins.
Jostine Joby, Yulia Marom, Guocong Lin, Aleksandra Baron‐Wiechec, Amit Meller   +4 more
wiley   +1 more source

Molecular Cross‐Linking of MXenes: Tunable Interfaces and Chemiresistive Sensing

Advanced Functional Materials, EarlyView.
In this study, Ti3C2Tx MXenes are initially functionalized using oleylamine ligands to form stable dispersions in an organic solvent. Subsequently ligand exchange with α,ω‐diaminoalkanes enables cross‐linking, along with precise tuning of interfaces. This structural control translates into tunable charge transport and responsive VOC sensing, showing ...
Yudhajit Bhattacharjee, Lukas Mielke, Mahmoud Al‐Hussein, Shivam Singh, Karen Schaefer, Borja Rodriguez‐Barea, Qiong Li, Anik Kumar Ghosh, Artur Erbe, Carmen Herrmann, Yana Vaynzof, Andreas Fery, Hendrik Schlicke   +12 more
wiley   +1 more source