Results 231 to 240 of about 362,057 (331)

Mitigating Singlet Exciton Back‐Transfer using 2D Spacer Layers for Perovskite‐Sensitised Upconversion

open access: yesAdvanced Optical Materials, EarlyView.
The efficiency of bulk perovskite‐sensitised upconversion is hindered by parasitic singlet back‐transfer. A 2D perovskite spacer layer is introduced to weaken this loss pathway by increasing the separation between the sensitiser and the emitter. The spacer layer enhances the upconversion efficiency at lower excitation powers and improves the stability ...
Nicholas P. Sloane   +10 more
wiley   +1 more source

Diameter Dependence of Light Absorption in GaAs Nanowires Evidenced by Photoluminescence Spectroscopy

open access: yesAdvanced Optical Materials, EarlyView.
Photoluminescence spectroscopy is introduced as a qualitative method to probe light absorption in highly phase‐pure GaAs nanowire arrays and single nanowires, for which direct absorption measurements are challenging. Using defect‐line saturation and the exciton‐to‐plasma transition as indicators for the density of photogenerated charge carriers, a ...
Francisca Marín   +3 more
wiley   +1 more source

Probing Ultrafast Coherent Bandgap Modulation in Monolayer WSe2 by Nonlinear Optics

open access: yesAdvanced Optical Materials, EarlyView.
This work sheds light on how resonant nonlinear optics blursthe line between perturbative and non‐perturbative nonlinear optics. Measured deviationsfrom the quadratic second‐harmonic scaling near the excitonic resonance arisefrom optical Stark and Bloch‐Siegert shifts. The experimental results arefurther underpinned by analytical and numerical analysis
Sebastian Klimmer   +7 more
wiley   +1 more source

Spectroscopic Ellipsometry Characterization and Radiative Limit Modeling of Bismuth‐Based Perovskite‐Inspired Absorbers for Indoor Photovoltaics

open access: yesAdvanced Optical Materials, EarlyView.
This study determines the optical constants of two lead‐free perovskite‐inspired materials (PIMs), Cu2AgBiI6 and Cs3Bi2I6Br3, promising for indoor light conversion. The optical constants are applied to simulate photovoltaic device optics, and thereupon, revise the theoretical limits for photocurrent generation and power conversion efficiency, providing
Aleksi Kamppinen   +6 more
wiley   +1 more source

Ultrabroadband Excitation of Hot Carriers in Plasmonic Nanorods Revealed by Two‐Dimensional Electronic Spectroscopy

open access: yesAdvanced Optical Materials, EarlyView.
This work dissects the ultrafast response of polydisperse plasmonic nanorods using two‐dimensional electronic spectroscopy, uniquely combining temporal and spectral resolution. Our ultrabroadband pulses cover both transverse and longitudinal nanorods’ resonances, revealing sub‐200‐fs dynamics and distinct broadening mechanisms.
Andrea Schirato   +8 more
wiley   +1 more source

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