Results 51 to 60 of about 1,368,587 (205)

Site Density Governs Switching Reactivity Regimes During Aerobic C─H Oxidation in Mn Single‐Atom Photocatalysts

Angewandte Chemie, EarlyView.
Increasing the density of isolated manganese (Mn) atoms in carbon nitride (CNx) photocatalysts does not continuously improve performance. Instead, beyond a critical loading, the polymer support reorganizes, altering charge‐carrier dynamics and oxygen activation while preserving atomic dispersion.
Viktoria Velichko, Agustín de Arriba, Areti Moutsiou, Elisabetta Inico, Andrea Olivati, Berta Pérez‐Román, Jesús López‐Sánchez, Ik Seon Kwon, Andrea Tonelli, Abhijit Roy, Valentina De Renzi, Raul Arenal, Annamaria Petrozza, Carlo Cavallotti, Gianvito Vilé   +14 more
wiley   +2 more sources

Generating Arbitrary Superpositions of Nonclassical Quantum Harmonic Oscillator States

Physical Review X
Full coherent control and generation of nonclassical superpositions of the quantum harmonic oscillator are not only of fundamental interest but are crucial for applications in quantum simulations, quantum-enhanced metrology, and continuous-variable ...
S. Saner, O. Băzăvan, D. J. Webb, G. Araneda, D. M. Lucas, C. J. Ballance, R. Srinivas   +6 more
doaj   +1 more source

Stretchable, Tough, and Luminescent Perovskite Molecular Ferroelectric Composite: Empowering Reliable Self‐Powered Motion Sensing in High Humidity and Subzero Temperatures

Advanced Science, EarlyView.
A flexible molecular ferroelectric composite is fabricated via in situ growth of luminescent DMAA‐MnCl3 ferroelectric crystals within a SEBS/SIS double‐polymer matrix. It delivers 7.54 MPa tensile strength, over 1200% tensile strain, durable piezoelectric motion sensing, and excellent harsh‐environment stability for all‐weather wearable biomechanical ...
Shuangqing Li, Zhe‐Kun Xu, Zheng Xing, Jin‐Wang Liu, Yong‐Quan Wu, Peng‐Fei Li, Zhong‐Xia Wang   +6 more
wiley   +1 more source

One‐Pot Biphasic Photocatalytic CO2‐to‐Carbonylation Cascades

Angewandte Chemie, EarlyView.
Bioinspired biphasic compartmentalization enables one‐pot cascades where photocatalytic CO2 reduction generates CO for carbonylative cross‐couplings to synthesize complex organic products, including a pharmaceutical. ABSTRACT Photosynthesis compartmentalizes reactions across the thylakoid membrane in vivo to upcycle CO2 into complex chemicals that are ...
Sampurna Mitra, David M. Vahey, Shannon A. Bonke, Erwin Reisner   +3 more
wiley   +2 more sources

Non-KAM classical chaos topology for electrons in superlattice minibands determines the inter-well quantum transition rates

Scientific Reports
We investigate the quantum-classical correspondence for a particle tunnelling through a periodic superlattice structure with an applied bias voltage and an additional tilted harmonic oscillator potential.
F. Wang, M. T. Greenaway, A. G. Balanov, T. M. Fromhold   +3 more
doaj   +1 more source

Laser Cooling of an Optomechanical Crystal Resonator to Its Quantum Ground State of Motion [PDF]

, 2012
Quantum mechanics continues to intrigue us with bizarre predictions that seemingly run counter to our everyday classical intuition. Superposition, zero-point motion, entanglement, and inescapable bounds on measurement precision are just a few purely ...
Chan, Jasper
core   +1 more source

Space‐Time Metasurface Antenna Enabled High‐Dimensional Electromagnetic Modulation for Intrinsic Physical Layer Security

Advanced Science, EarlyView.
The concept of high‐dimensional EM modulation using the STMA for physical layer secure communication is illustrated in figure. The STMA consists of a series of programmable unit cells, with 1‐bit reconfigurable phase states (0/π). The STMA is excited by a monochromatic continuous wave (CW) at frequency fc and controlled by a field‐programmable gate ...
Xinyu Fang, Yiqing Sun, Chenfeng Yang, Siran Wang, Zheng Xing Wang, Kaixu Wang, Geng‐Bo Wu   +6 more
wiley   +1 more source

Axially Chiral Nonalternant Polycyclic Aromatic Hydrocarbon With Consecutive Pentagons Exhibiting Large Spin‐Polarized Current

Angewandte Chemie, EarlyView.
Here we report two nonalternant polycyclic aromatic hydrocarbons (PAH) (1 and 2), which contain two and four consecutive pentagons, respectively. Under acidic conditions, 1 and 2 dimerize to afford the axially chiral dimers AC1 and AC2. The central azulene moiety in both 2 and AC2 shows an unusually short transannular bond of 1.366 Å.
Chang Wang, Jiaxin Luo, Haipeng Lu, Junzhi Liu   +3 more
wiley   +2 more sources

Evaluating the performance of classical, quantum, and hybrid quantum neural networks in solving differential equations

Scientific Reports
We investigate the performance of classical, quantum, and hybrid quantum neural networks in solving partial differential equations through both supervised and unsupervised learning.
Navid Markazi, Behrouz Mirza
doaj   +1 more source

Many body effects in one-dimensional attractive Bose gases [PDF]

, 2013
In this thesis we investigate the properties of ultra-cold quantum gases in reduced dimension and the effects of harmonic confinement on soliton-like properties.
HOLDAWAY, DAVID,IAN,HENRY
core