Results 181 to 190 of about 2,788 (253)

Parity‐Dependent THz Harmonic Generation in Electrically Pumped Micro‐Lasers Exploiting Topological Insulator–Metamaterial Gratings

open access: yesAdvanced Materials, EarlyView.
Topological insulator–metamaterials integrated with electrically driven terahertz quantum cascade lasers enable parity‐dependent harmonic generation. Bulk‐dominated Bi2Se3 favors third‐harmonic emission at 9.96 THz, whereas topological‐surface‐state‐dominated Bi2Se3, Bi2Te3, and (Bi,Sb)2Te3 generate strong second harmonics near 6.5 THz.
Alessandra Di Gaspare   +9 more
wiley   +1 more source

Phase‐Engineered MoS2 Quantum Monolayer Catalysts

open access: yesAdvanced Materials, EarlyView.
A new type of catalyst model—phase‐engineered MoS2 quantum‐monolayer catalyst (∼0.8 nm thick, < 6 nm in the lateral size; switchable freely among metallic 1T, semiconducting 2H, and a hybrid phase of metallic‐semiconducting 1T‐2H)—is reported. It can efficiently and stably drive photochemical H2, syngas and ammonia synthesis as a catalyst or co ...
Ruijie Yang   +12 more
wiley   +1 more source

Efficient in‐Plane Exciton Transport in a Discontinuous Layered Lead‐Bromide Perovskite

open access: yesAdvanced Materials, EarlyView.
A new class of two‐dimensional lead‐bromide perovskite based on monovalent 4‐aminomethylbenzoic acid cations is presented, featuring a discontinuous inorganic layer. Despite the discontinuous lattice, transient photoluminescence microscopy demonstrates efficient though strongly anisotropic in‐plane exciton transport.
Raquel Utrera‐Melero   +9 more
wiley   +1 more source

In Situ Formation of a Highly Selective Nickel Single Atom Catalyst for Electrochemical CO2 Reduction to CO

open access: yesAdvanced Materials, EarlyView.
Development of a novel method for synthesizing Ni single atom catalysts for highly selective electrochemical CO2 reduction in situ. This catalyst achieves 100% selectivity for CO and is formed in an industrially relevant cell architecture. Using post‐mortem XRD, STEM, and EDS and operando XAS, the identity of the active site and the mechanism behind ...
Ian Street   +5 more
wiley   +1 more source

Highly Sensitive Broadband Photodetectors Based on Donor–Acceptor 2D Conjugated Coordination Polymers

open access: yesAdvanced Materials, EarlyView.
Donor–acceptor molecular design and chemical vapor deposition growth enable the two‐dimensional nickel‐tetraaminobenzoquinone films with strong broadband absorption and efficient charge separation. The resulting photodetectors exhibit a structured broadband response with a high responsivity of ∼3.1 A W−1 and a response time of ∼170 µs, which surpasses ...
Yunxu Chen   +14 more
wiley   +1 more source

Quantum-Centric Alchemical Free Energy Calculations. [PDF]

open access: yesJ Chem Theory Comput
Bazayeva M   +6 more
europepmc   +1 more source

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