Results 91 to 100 of about 60,354 (258)

On‐Surface Indigo‐Based Bimolecular Coordination Networks with Programmable Regular or Vitreous Structure

open access: yesAdvanced Functional Materials, EarlyView.
A previously unreported coordination motif stabilising single Fe atoms by indigo chelation and pyridyl coordination on Au(111) has been revealed. By using planar tritopic pyridyl linkers (TPyB), extended 2D porous networks of indigo3(TPyB)2Fe6 form. These networks can be crystalline or vitreous and offer an environment where individual coordination ...
Hongxiang Xu   +9 more
wiley   +1 more source

MOFs and COFs in Electronics: Bridging the Gap between Intrinsic Properties and Measured Performance

open access: yesAdvanced Functional Materials, EarlyView.
Metal‐organic frameworks (MOFs) and covalent organic frameworks (COFs) hold promise for advanced electronics. However, discrepancies in reported electrical conductivities highlight the importance of measurement methodologies. This review explores intrinsic charge transport mechanisms and extrinsic factors influencing performance, and critically ...
Jonas F. Pöhls, R. Thomas Weitz
wiley   +1 more source

Process tomography of structured optical gates with convolutional neural networks

open access: yesMachine Learning: Science and Technology
Efficient and accurate characterization of an experimental setup is a critical requirement in any physical setting. In the quantum realm, the characterization of an unknown operator is experimentally accomplished via Quantum Process Tomography (QPT ...
Tareq Jaouni   +4 more
doaj   +1 more source

Auto‐Generated Valence States in Electrocatalysts for Boosting Oxygen and Hydrogen Evolution Kinetics in Alkaline Water/Alkaline Seawater/Simulated Seawater/Natural Seawater

open access: yesAdvanced Functional Materials, EarlyView.
This review systematically highlights the latest achievements in mixed‐valence states relevant to hydrogen and oxygen evolution reactions, providing essential insights into future directions and methods for large‐scale practical implementation. This critical review is expected to provide an overview of recent advancements in diverse valence‐state metal
Jitendra N. Tiwari   +4 more
wiley   +1 more source

DNA‐Templated 2D Heterostructures as Phototriggered Dynamic Nanohybrids: From Releasing Molecular Loads to Controlling Enzyme Biocatalytic Function

open access: yesAdvanced Functional Materials, EarlyView.
DNA strands are employed both as dynamic linkers and nanoscale templates for the integration of Ag2S nanoparticles on MoS2, which in turn imparted photothermal responsiveness; this feature permits the selective cargo (fluorophore, quantum dots or an enzyme) release from the MoS2 surface in response to local heat induced by light irradiation.
Kai Chen   +3 more
wiley   +1 more source

Quantum tomography of input-output processes [PDF]

open access: yesPhysical Review A, 2000
We demonstrate the possibility of practical tomographic determination of arbitrary input-output transformations. It is shown that the Liouville-space formalism provides a generalization of standard tomography encompassing the reconstruction of processes as well as of quantum states.
openaire   +3 more sources

Slight Truncation Changes in Iron Oxide Nanocubes Strongly Affect Their Magnetic Properties

open access: yesAdvanced Functional Materials, EarlyView.
Subtle variations in nanoparticle morphology can lead to significant changes in functional properties. An automated shape‐fitting method captures minor differences in corner truncation between iron oxide nanocubes of similar sizes synthesized under identical conditions, revealing pronounced disparities in their magnetic and hyperthermia behavior ...
Kingsley Poon   +7 more
wiley   +1 more source

Quantum process identification: a method for characterizing non-markovian quantum dynamics

open access: yesNew Journal of Physics, 2019
Established methods for characterizing quantum information processes do not capture non-Markovian (history-dependent) behaviors that occur in real systems.
Ryan S Bennink, Pavel Lougovski
doaj   +1 more source

Learning Quantum Processes with Quantum Statistical Queries [PDF]

open access: yesQuantum
In this work, we initiate the study of learning quantum processes from quantum statistical queries. We focus on two fundamental learning tasks in this new access model: shadow tomography of quantum processes and process tomography with respect to diamond
Chirag Wadhwa, Mina Doosti
doaj   +1 more source

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