Vibronic effects on the quantum tunnelling of magnetisation in Kramers single-molecule magnets [PDF]
Nature Communications, 2023 Single-molecule magnets are among the most promising platforms for achieving molecular-scale data storage and processing. Their magnetisation dynamics are determined by the interplay between electronic and vibrational degrees of freedom, which can couple
Andrea Mattioni +6 more
doaj +4 more sources
Unraveling the Contributions to Spin-Lattice Relaxation in Kramers Single-Molecule Magnets. [PDF]
J Am Chem Soc, 2022 The study of how spin interacts with lattice vibrations and relaxes to equilibrium provides unique insights into its chemical environment and the relation between electronic structure and molecular composition.
Mondal S, Lunghi A.
europepmc +2 more sources
Lanthanide single-molecule magnets with high anisotropy barrier: where to from here? [PDF]
Natl Sci Rev, 2022 High-temperature lanthanide single-molecule magnets with large coercive fields are being pursued.
Zhu Z, Tang J.
europepmc +2 more sources
Coupling single-molecule magnets to quantum circuits [PDF]
New Journal of Physics, 2013 In this work we study theoretically the coupling of single-molecule magnets (SMMs) to a variety of quantum circuits, including microwave resonators with and without constrictions and flux qubits.
Mark Jenkins +5 more
doaj +4 more sources
Single-molecule magnets beyond a single lanthanide ion: the art of coupling. [PDF]
Chem Sci, 2022 The promising future of storing and processing quantized information at the molecular level has been attracting the study of Single-Molecule Magnets (SMMs) for almost three decades.
Chen YC, Tong ML.
europepmc +2 more sources
Spin-phonon coupling and magnetic relaxation in single-molecule magnets.
Chem Soc Rev, 2023 Electron–phonon coupling is important in many physical phenomena, e.g. photosynthesis, catalysis and quantum information processing, but its impacts are difficult to grasp on the microscopic level.
Kragskow JGC +5 more
europepmc +2 more sources
Quantum turnstile operation of single-molecule magnets [PDF]
New Journal of Physics, 2015 The time-dependent transport through single-molecule magnets coupled to magnetic or non-magnetic electrodes is studied in the framework of the generalized master equation method.
V Moldoveanu +3 more
doaj +3 more sources
Mononuclear Dysprosium Alkoxide and Aryloxide Single-Molecule Magnets. [PDF]
Chemistry, 2021 Recent studies have shown that mononuclear lanthanide (Ln) complexes can be high‐performing single‐molecule magnets (SMMs). Recently, there has been an influx of mononuclear Ln alkoxide and aryloxide SMMs, which have provided the necessary geometrical ...
Parmar VS, Mills DP, Winpenny REP.
europepmc +2 more sources
A Cost-Effective Semi-Ab Initio Approach to Model Relaxation in Rare-Earth Single-Molecule Magnets. [PDF]
J Phys Chem Lett, 2021 We discuss a cost-effective approach to understand magnetic relaxation in the new generation of rare-earth single-molecule magnets. It combines ab initio calculations of the crystal field parameters, of the magneto-elastic coupling with local modes, and ...
Garlatti E +16 more
europepmc +2 more sources
The Separation of the Mn12 Single-Molecule Magnets onto Spherical Silica Nanoparticles [PDF]
Nanomaterials, 2019 The Mn12 single-molecule magnets (SMMs) could be attached to the surface of spherical silica for the first time with a high probability. This allowed separation of the individual molecular magnets and direct microscopic observation of the SMMs.
Lukasz Laskowski +5 more
doaj +2 more sources