Machine learning force field ranking of candidate solid electrolyte interphase structures in Li-ion batteries [PDF]
, 2023 The Solid-Electrolyte Interphase (SEI) formed in lithium-ion batteries is a vital but poorly-understood class of materials, combining organic and inorganic components.
James, Stevenson +2 more
core +1 more source
Kinetically corrected Monte Carlo-molecular dynamics simulations of solid electrolyte interphase growth [PDF]
, 2021 We present a kinetic approach to the Monte Carlo-molecular dynamics (MC-MD) method for simulating reactive liquids using non-reactive forcefields. A graphical reaction representation allows definition of reactions of arbitrary complexity, including their
Joseph W, Abbott, Felix, Hanke
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Towards a Mechanistic Model of Solid-Electrolyte Interphase Formation and Evolution in Lithium-ion Batteries [PDF]
, 2022 The formation of passivation films by interfacial reactions, though critical for applications ranging from advanced alloys to electrochemical energy storage, is often poorly understood.
Ronald L, Kam +7 more
core +2 more sources
Effect of current density on the Li – Li6PS5Cl solid electrolyte interphase [PDF]
, 2022 Understanding the nature and evolution of interphasial products at the Li metal – solid electrolyte interface is crucial in solid-state lithium batteries (SSBs).
Yvonne, Chart +5 more
core +2 more sources
Operando characterization and theoretical modelling of metal|electrolyte interphase growth kinetics in solid-state-batteries - Part II: Modelling [PDF]
, 2022 Understanding the interfacial dynamics of batteries is crucial to control degradation and increase electrochemical performance and cycling life. If the chemical potential of a negative electrode material lies outside of the stability window of an ...
Nicholas J., Williams +4 more
core +2 more sources
Operando characterization and theoretical modelling of metal|electrolyte interphase growth kinetics in solid-state-batteries - Part I: experiments [PDF]
, 2022 To harness all the benefits of solid-state battery (SSB) architectures in terms of energy density, their negative electrode should be an alkali metal.
Nicholas J., Williams +4 more
core +2 more sources
Advanced Science, 2023 Argyrodite‐type Li6PS5Cl (LPSCl) has attracted much attention as a solid electrolyte for all‐solid‐state batteries (ASSBs) because of its high ionic conductivity and good mechanical flexibility. LPSCl, however, has challenges of translating research into
Kanghyeon Kim +7 more
doaj +1 more source
Constructing a Quasi-Liquid Interphase to Enable Highly Stable Zn-Metal Anode
Batteries, 2023 Rechargeable aqueous Zn-metal batteries have attracted widespread attention owing to their safety and low cost beyond Li-metal batteries. However, due to the lack of the solid electrolyte interphase, problems such as dendrites, side reactions and ...
Junzhang Wang +8 more
doaj +1 more source
Revealing Solid Electrolyte Interphase Formation Through Interface-Sensitive Operando X-ray Absorption Spectroscopy [PDF]
, 2022 The solid electrolyte interphase (SEI) that forms on Li-ion battery anodes is critical to their long-term performance, however observing SEI forma- tion processes at the buried electrode-electrolyte interface is a significant challenge. Here we show that
Clare, Grey +12 more
core +2 more sources
High‐Efficacy and Polymeric Solid‐Electrolyte Interphase for Closely Packed Li Electrodeposition
Advanced Science, 2021 The industrial application of lithium metal anode requires less side reaction between active lithium and electrolyte, which demands the sustainability of the electrolyte‐induced solid‐electrolyte interface.
Siyuan Li +10 more
doaj +1 more source