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Proximity Matters: Interfacial Solvation Dictates Solid Electrolyte Interphase Composition
Nano Letters, 2023The composition of the solid electrolyte interphase (SEI) plays an important role in controlling Li-electrolyte reactions, but the underlying cause of SEI composition differences between electrolytes remains unclear. Many studies correlate SEI composition with the bulk solvation of Li ions in the electrolyte, but this correlation does not fully capture
Solomon T. Oyakhire +9 more
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Molecularly Woven Artificial Solid Electrolyte Interphase
Angewandte ChemieAbstract Lithium‐metal batteries (LMBs) are the most promising candidates for next‐generation high‐energy‐density storage systems, but they suffer from destructive dendrite growth. Here, we integrate cutting‐edge molecular weaving technology into the fabrication of artificial solid electrolyte interphases (ASEI ...
Tianyu Shan +10 more
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Solid Electrolyte Interphase on Lithium Metal Anodes
ChemSusChemAbstractLithium metal batteries (LMBs) represent the most promising next‐generation high‐energy density batteries. The solid electrolyte interphase (SEI) film on the lithium metal anode plays a crucial role in regulating lithium deposition and improving the cycling performance of LMBs. In this review, we comprehensively present the formation process of
Zhichuan Shen +5 more
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Solid-Electrolyte-Interphase: Characterization by Impedance Spectroscopy
ECS Meeting Abstracts, 2009Abstract not Available.
George Harriott +4 more
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Single-Component Solid Electrolyte Interphases on Lithium
ECS Meeting Abstracts, 2019The ability to utilize Li metal anodes in rechargeable batteries would be an enabling breakthrough in the quest to increase energy density and meet current aggressive performance targets (> 350 Wh/kg) for electric vehicles. However, Li anodes face several persistent challenges:1 ,2 (1) Large volume expansion upon cycling, leading
Betar M. Gallant, Mingfu He, Rui Guo
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Protective Oxide Coating for Ionic Conductive Solid Electrolyte Interphase
ACS Applied Materials & Interfaces, 2016To employ Li-based batteries to their full potential in a wide range of energy-storage applications, their capacity and performance stability must be improved. Si is a viable anode material for Li-based batteries in electric vehicles due to its high theoretical capacity and good economic feasibility.
Yong Su, Kim +10 more
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Structural Properties of Solid Electrolyte Interphase on Lithium Metal
Journal of Nanoscience and Nanotechnology, 2015To gain an understanding of the structural properties of the solid electrolyte interphase (SEI) created on the surface of lithium during an electrochemical deposition/dissolution reaction in propylene carbonate (PC) containing different concentrations of LiClO4 (1.09, 3.27 mol kg(-1)), the surface of lithium was examined through transmission electron ...
Soon-Ki, Jeong +2 more
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In Situ and Quantitative Characterization of Solid Electrolyte Interphases
Nano Letters, 2014Despite its importance in dictating electrochemical reversibility and cell chemistry kinetics, the solid electrolyte interphase (SEI) on graphitic anodes remains the least understood component in Li ion batteries due to its trace presence, delicate chemical nature, heterogeneity in morphology, elusive formation mechanism, and lack of reliable in situ ...
Arthur, v Cresce +4 more
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Breakthrough on understanding the solid electrolyte interphase
Science Bulletin, 2022Shihan, Qi, Xiu, Li, Jianmin, Ma
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Regulating Li deposition at artificial solid electrolyte interphases
Journal of Materials Chemistry A, 2017An artificial solid electrolyte interphases (SEI) layer was established on the lithium metal anode via magnetron sputtering deposition for promoting uniform lithium electrodeposition.
Lei Fan +4 more
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