Balancing Electrons to Break the Activity‐Selectivity Trade‐Off in H2O2 Electrosynthesis
Carrier‐concentration balancing in CuS is achieved by coupling cobalt dopants with cobalt vacancies, converting CuS from p‐ to n‐type to accelerate 2e− ORR while withdrawing excess carriers to optimize *OOH binding for H2O2 desorption. The catalyst reaches 8.14 mol g−1 h−1 with >84% selectivity in 1.0 M KOH and drives robust electro‐Fenton dye ...
Hangning Liu +11 more
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Comprehensive Study of Li Deposition and Solid Electrolyte Cracking by Integrating Simulation and Experimental Data. [PDF]
Lin C, Ruan H, Wang MS.
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This work introduces a regionally localized electrolyte (RLE) that spatially separates ether‐ and carbonate‐based functions to stabilize both Li metal and high‐voltage cathodes. An immobilized ether‐rich layer directs Li+ transport, activates LiNO3 locally, and forms a uniform LiF‐rich SEI, enabling lower overpotential, uniform deposition, and long ...
Eunbin Lim +4 more
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Artificial Solid Electrolyte Interphase Developed In Vitro by Tailoring Molecular Layer Deposition of a Li-Ion-Containing Electrolyte on Carbonaceous Anode Materials. [PDF]
Fedorov RG +7 more
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A tandem gas diffusion electrode (GDE) leveraging hierarchically engineered microgranules enables efficient CO2 electroreduction under dilute CO2 conditions. A key innovation lies in the solvent‐free precision assembly of metal–organic‐frameworks, carbon nanotubes, and copper nanoparticles.
Kai‐Jen Wu +7 more
wiley +1 more source
Formation and Evolution of the Solid Electrolyte Interphase on Silicon Electrodes from Fluorine-Free Electrolytes. [PDF]
Lu Z +6 more
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Electrochemical CO2 reduction (ECR) to formate is a promising route for sustainable chemical production. Herein, we report the synthesis catalysed byBi‐HfO2@C. The AIMD simulations, DFT calculations, and in situ SEIRAS measurements show that the modification of HfO2 on the Bi surface steers the interfacial water to adopt a favorable hydrogen‐down (OH2↓)
Xiao‐Dong Guo +7 more
wiley +1 more source
Pre-Constructed Mechano-Electrochemical Adaptive Solid Electrolyte Interphase to Enhance Li<sup>+</sup> Diffusion Kinetics and Interface Stability for Chemically Prelithiated SiO Anodes. [PDF]
Wang Z +10 more
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Eutectic-Like Ion-Conductive Phase-Incorporated Zwitterionic Covalent Organic Framework Solid Electrolyte for All-Solid-State Li Metal Batteries. [PDF]
Lee J +8 more
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Revealing the roles of the solid-electrolyte interphase in designing stable, fast-charging, low-temperature Li-ion batteries. [PDF]
Tao L +18 more
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