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The role of phosphorus in the solid electrolyte interphase of argyrodite solid electrolytes [PDF]

open access: yesNature Communications
The solid electrolyte interphase that forms on Li6PS5Cl argyrodite solid electrolytes has been reported to continually grow through a diffusion-controlled process, yet this process is not fully understood.
Matthew Burton   +8 more
doaj   +2 more sources

De-solvation of heteroalkali cations enabling stable solid electrolyte interphase for dendrite-free lithium metal batteries [PDF]

open access: yesNature Communications
Li metal is highly sought after as a negative electrode material due to its high specific capacity and low electrode potential. However, the brittle solid electrolyte interphase and undesirable coulombic efficiency have severely hindered its commercial ...
Aoyuan Chen   +7 more
doaj   +2 more sources

Solid electrolyte interphase in water-in-salt electrolytes [PDF]

open access: yesScience China Materials, 2021
The water-in-salt strategy successfully expands the electrochemical window of the aqueous electrolyte from 1.23 to ∼3.0 V, which can lead to a breakthrough in the energy output of the aqueous battery system while maintaining the advantage of high safety.
Dezhong Liu, Lixia Yuan, Yunhui Huang
openaire   +1 more source

Nanoarchitecture factors of solid electrolyte interphase formation via 3D nano-rheology microscopy and surface force-distance spectroscopy

open access: yesNature Communications, 2023
Characterization of the solid electrolyte interphase formed on Li-ion battery electrodes presents significant experimental challenges. Here the authors use atomic force microscopy-based force-spectroscopy techniques to depict the initial interphase ...
Yue Chen   +13 more
doaj   +1 more source

An electrochemically stable homogeneous glassy electrolyte formed at room temperature for all-solid-state sodium batteries

open access: yesNature Communications, 2022
Single sodium-ion solid electrolyte that meets the requirements of practical applications is difficult to design. Here, the authors show how kinetic stability via the creation of a self-passivating solid electrolyte interphase allows a homogenous glass ...
Xiaowei Chi   +15 more
doaj   +1 more source

Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries

open access: yesInorganics, 2022
Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone.
Dominic Spencer Jolly   +11 more
doaj   +1 more source

Phase-Field Computational Framework for Addressing Challenges in Solid-State Batteries

open access: yesPRX Energy, 2023
All-solid-state batteries are attracting increasing interest due to their higher promised energy densities without the use of flammable liquid electrolytes.
Tammo K. Schwietert   +9 more
doaj   +1 more source

Constructing a Quasi-Liquid Interphase to Enable Highly Stable Zn-Metal Anode

open access: yesBatteries, 2023
Rechargeable aqueous Zn-metal batteries have attracted widespread attention owing to their safety and low cost beyond Li-metal batteries. However, due to the lack of the solid electrolyte interphase, problems such as dendrites, side reactions and ...
Junzhang Wang   +8 more
doaj   +1 more source

Trimethylsilyl Compounds for the Interfacial Stabilization of Thiophosphate‐Based Solid Electrolytes in All‐Solid‐State Batteries

open access: yesAdvanced Science, 2023
Argyrodite‐type Li6PS5Cl (LPSCl) has attracted much attention as a solid electrolyte for all‐solid‐state batteries (ASSBs) because of its high ionic conductivity and good mechanical flexibility. LPSCl, however, has challenges of translating research into
Kanghyeon Kim   +7 more
doaj   +1 more source

High‐Efficacy and Polymeric Solid‐Electrolyte Interphase for Closely Packed Li Electrodeposition

open access: yesAdvanced Science, 2021
The industrial application of lithium metal anode requires less side reaction between active lithium and electrolyte, which demands the sustainability of the electrolyte‐induced solid‐electrolyte interface.
Siyuan Li   +10 more
doaj   +1 more source

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