Results 141 to 150 of about 17,751 (261)

Sensitive and Spatially‐Resolved Electrochemiluminescence via Micropatterning

Advanced Materials Interfaces, EarlyView.
The use of a simple silica nanoparticle surface coating and patterning process can transform ordinary gold electrodes into multiplexed ECL sensing electrodes. Through spatially confined droplet formation and local ECL emission, it is possible to perform multiple analyses simultaneously from individual locations as well as intensify the ECL signal by as
Yuliang Shao, Tatiana Starikova, Mengzhen Xi, Maria Vittoria Balli, Emanuele Luigi Sciuto, Gabriele Giagu, Vincenzo Paratore, Carmelo Corsaro, Enza Fazio, Sabrina Conoci, Luca Prodi, Giovanni Valenti, Pavel A. Levkin   +12 more
wiley   +1 more source

Shadow‐Free Back‐Contact Perovskite Thin‐Film Detectors for Direct Extreme‐Ultraviolet and Soft X‐Ray Sensing

Advanced Materials Interfaces, EarlyView.
A triple‐cation perovskite detector with a quasi‐interdigitated back‐contact architecture enables highly sensitive and linear EUV/soft x‐ray detection by minimizing electrode shadowing and enhancing charge extraction. Efficient interfacial carrier collection and rapid temporal response highlight the potential of back‐contact‐engineered perovskites for ...
Jingying Liu, Siqi Deng, Mosarof Hossain, Udo Bach, Kaijian Xing, Qingdong Ou   +5 more
wiley   +1 more source

Femtosecond X-ray photon correlation spectroscopy enables direct observations of atomic-scale relaxations of glass forming liquids

Glass-forming liquids exhibit structural relaxation behaviors, reflecting underlying atomic rearrangements on a wide range of timescales and playing a crucial role in determining material properties.
Moesgaard, Jens, Albert, Thies, Wang, Nan, Esposito, Vincent, Li, Haoyuan, Chen, Ying, Fuoss, Paul, David, Christian, Mo, Mianzhen, Fujita, Tomoki, Sato, Takahiro, Sun, Peihao, Albert, Thies J, Mamyrbayev, Talgat, Sokolowski-Tinten, Klaus, Ruta, Beatrice, Hastings, Jerome, Amini, Narges, Zhu, Diling, Yang, Fan, Lucas, Pierre, Vila-Comamala, Joan, Sun, Yanwen, Wei, Shuai, Song, Sanghoon, Cornet, Antoine   +25 more
core   +1 more source

Fast two-dimensional detection for X-ray photon correlation spectroscopy using the PILATUS detector

, 2009
International audienceThe first X-ray photon correlation spectroscopy experiments using the fast single-photon-counting detector PILATUS (Paul Scherrer Institut, Switzerland) have been performed.
Duri, Agnès, Grübel, G., Broennimann, C., Autenrieth, T., Westermeier, F., Gutt, C., Leupold, O., Johnson, I., Menzel, A.   +8 more
core   +1 more source

Benchmarking Coaxial and Angular Optical Emission Spectroscopy With Recommendations for Reliable Compositional In Situ Monitoring During Laser Powder Bed Fusion

Advanced Materials Technologies, EarlyView.
ABSTRACT Real‐time insight into local chemistry is critical for reliable part quality in additive manufacturing, especially laser powder bed fusion (PBF‑LB/M), where rapid thermal cycles and localized evaporation can undermine part performance. Optical emission spectroscopy (OES) offers non‑intrusive, in situ plume monitoring, but detection geometry ...
Philipp Gabriel, Bastian Jülich, Anna Rosa Ziefuss, Florian Eibl, Stephan Barcikowski   +4 more
wiley   +1 more source

The Influence of Mesoscale Particle Structure on the Electrode Degradation and Resultant Electrochemistry of Lithium Ion Cells With Nickel Rich Lithium Nickel Manganese Cobalt Oxide Positive Electrodes

Advanced Materials Technologies, EarlyView.
Milled polycrystalline NMC811 cathode (MPC NMC) with smaller secondary particle and higher surface area had 1) greater cathode tortuosity, 2) reduced surface Ni on the cycled MPC cathodes consistent with surface reconstruction, and 3) increased Ni deposition from cathode‐anode crosstalk, manifesting in lower functional capacity and higher impedance ...
Edelmy J. Marin Bernardez, Andrew Nicoll, David J. Arnot, Armando Rodriguez Campos, Patrick J. Barry, Marie F. Millares, Cynthia Huang, Melissa A. Guercio, Grace K. Dono, Alexis Pace, Xianghui Xiao, Cherno Jaye, Conan Weiland, Jianming Bai, Hui Zhong, Michael Drakopoulos, Zhong Zhong, Nghia T. Vo, Xiao Tong, Esther S. Takeuchi, Amy C. Marschilok, Shan Yan, Kenneth J. Takeuchi   +22 more
wiley   +1 more source

High‐Power Rapid Laser‐Induced Synthesis of Multi‐functional Cobalt Metal‐Organic Framework With an Unprecedented Synthesis Efficiency

Advanced Materials Technologies, EarlyView.
Laser‐assisted synthesis enables rapid (within 1 h) and high‐yield (≥90%) production of Co‐MOFs with mesoporous structures, tunable magnetic and optical properties, and efficient adsorption of N2, CH4, and CO2 for low‐energy gas separation. DFT calculations elucidate the electronic structure and adsorption behavior.
Saliha Mutlu, Bülend Ortaç, Ali Karatutlu, Taylan Gorkan, Engin Durgun, Dilek Soyler, Saniye Soylemez, Jelena Lillepäg, Volkan Filiz, Nergis Arsu, Sevil Savaskan Yilmaz   +10 more
wiley   +1 more source

Highly Anisotropic Quasi‐Direct Organic Metal Halide Hybrids: A Platform for Polarization‐Sensitive Optoelectronics

Advanced Materials Technologies, EarlyView.
One‐dimensional C4N2H14PbBr4 is shown to have a quasi‐direct electronic band structure and strongly anisotropic transport with polarized broadband emission. A GW/Bethe–Salpeter excited‐state force formalism, supported by polarized Raman and temperature‐dependent photoluminescence, identifies low–frequency Pb–Br phonons that drive ultrafast exciton self‐
Rijan Karkee, Rafael R. Del Grande, Yeonjoo Lee, Jinkyoung Yoo, Azza Ben‐Akacha, Biwu Ma, Michael T. Pettes, David A. Strubbe   +7 more
wiley   +1 more source

Linking Device Performance to Nanoscale Photoactivation of Grain Boundaries in 2D Hybrid Halide Perovskites

Advanced Materials Technologies, EarlyView.
The opto‐electronic response of polycrystalline (PEA)2PbBr4 thin films is investigated by correlating macroscopic photodetector performance with nanoscale mapping techniques. Grain boundary density is systematically tuned through crystallization control and linked to device responsivity.
Camilla Bordoni, Lorenzo Calcaterra, Andrea Ciavatti, Silvia Milita, Valentina Bonino, Lorenzo Margotti, Sara Cepić, Marisa Di Sabatino, Federico Boscherini, Daniela Cavalcoli, Beatrice Fraboni   +10 more
wiley   +1 more source

Thickness‐Dependent Infrared Emissivity of Ultrathin Freestanding MoSiN Nanocomposite Membranes

Advanced Optical Materials, EarlyView.
ABSTRACT Metals and dielectrics show opposite trends in thickness‐dependent infrared emissivity: metallic films exhibit a rise in emissivity below a critical thickness, while dielectric films show a corresponding decline. For applications demanding both high emissivity and mechanical strength in membranes with nanoscale thickness, combining these ...
Reethu Sebastian, Amrid Amnache, Nadi Braidy, Luc G. Fréchette   +3 more
wiley   +1 more source