Results 41 to 50 of about 4,178 (175)
在种还分离模式下采用尼龙网袋法对玉米秸秆还田进行田间原位模拟,比较不同秸秆还田量在不同还田深度下对土壤总有机碳、微生物量碳、纤维素酶活性和过氧化氢酶活性的影响。试验设置秸秆还田量0(R0),0.44%(R1),0.88%(R2)和1.32%(R3)4个水平和3个还田深度0—15,15—30,30—45 cm交叉处理。结果表明:还田1年时,在0—15 cm土层,土壤总有机碳、微生物量碳、纤维素酶活性和过氧化氢酶活性均随秸秆还田量增加而提高,且R3处理提升效果最显著,分别达到30.98%,101.16 ...
刘 龙, 李志洪, 赵小军, 崔婷婷
doaj
活性碳上羧酸根锚定AuCl3催化乙炔氢氯化反应的理论研究 [PDF]
采用密度泛函B3LYP方法,运用分子模型对活性碳(AC)上羧酸根负载AuClx催化剂的活性结构、稳定性以及催化乙炔氢氯化反应机制进行了详细的理论探讨。结果表明,AuCl3催化剂可以被表面羧酸根单中心级分散锚定,形成AC-COOH-AuCl3表面活性中心,进而在氢氯化过程中与乙炔发生协同加成生成氯乙烯,同时形成具有螯合结构的表面活性中心AC-CO2>AuCl2,进而催化氢氯化反应遵循分步反应异步加成机制:乙炔活化吸附到Au(Ⅲ)中心,HCl异裂亲核加成到乙炔伴随羧酸根质子化,分子内质子迁移形成Au(Ⅲ ...
吕鑫, 宁利超, 张冠如, 谭凯
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Cu‐Based Catalysts Design Toward Electrochemical CO2 Reduction to Valuable Multi‐Carbons Products
ABSTRACT Electrochemical reduction of CO2 to multi‐carbon products (e.g., C2+, ethene, ethanol, etc.) not only effectively decreases the CO2 concentration in atmosphere but also shows great potential economic benefits due to these exploitable value‐added products. The Cu‐based catalysts have caught much attention in CO2 electroreduction due to the good
Li‐Qing Li +5 more
wiley +1 more source
对若尔盖高寒湿地沼泽土和泥炭土的有机碳(TOC)和活性有机碳(LC)沿土壤剖面的分布特征研究表明,沼泽土的有机碳和全氮(TN)古量整体上从表层向下呈现下降趋势.中间在16~18cm处出现一个升高点,与当时的有机质来源和沉积环境有关。泥炭土有机碳沿土壤剖面并没有呈现同样的下降趋势.而是从表层向下至22cm呈现升高趋势,22cm向下才呈现下降趋势。全氮含量与有机碳含量的分布特征不同。在表层o~10cm古量较高,向下含量减小。沼泽土活性有机碳沿土壤剖面整体呈现下降趋势,变化于2.4~13.6mg/g ...
高俊琴, 欧阳华, 白军红
doaj
Creating the future for a better world [PDF]
WFF is a grant-making foundation, based in Singapore, but for the world. It provides financial support to a number of organizations and programs related to environmental and social sustainability research. Through these programs, WFF hopes to bring forth
core
ABSTRACT Prelithiation is effective for compensating active lithium‐ion (Li+) loss in silicon (Si)‐based battery electrode materials. However, owing to the dynamic growth of the solid electrolyte interface (SEI), capacity fading remains the biggest challenge for the industrialization of Si electrodes.
Wen‐Jie He +9 more
wiley +1 more source
为探究闽江口湿地土地利用和恢复对土壤酶活性的影响,采集闽江口芦苇湿地、滩涂地、草地、农田和撂荒地5种不同土地利用方式,分析土壤β—葡萄糖苷酶、N—乙酰—氨基葡萄糖苷酶、L—亮氨酸—氨基肽酶和酸性磷酸酶活性及与环境因子之间的关系。结果表明:土壤pH、铵态氮和硝态氮在农田土壤显著高于其他土地利用方式;而土壤碳(C)、氮(N)、磷(P)全量含量在撂荒地和芦苇湿地显著高于其他土地利用方式。撂荒地、农田和芦苇湿地可溶性碳氮含量显著高于滩涂和草地土壤;土壤微生物量碳氮含量在不同土地利用方式间变化趋势比较一致 ...
刘子恺 +5 more
doaj
ABSTRACT Formic acid (FA) is considered to be a safe and convenient hydrogen source; however, achieving controlled and efficient FA dehydrogenation under mild conditions using stable solid catalysts remains a significant challenge. Pd‐based catalysts have been extensively studied due to their superior catalytic activity to other metal catalysts.
Shuai Wei +10 more
wiley +1 more source
ABSTRACT The development of novel oxygen electrocatalysts with cost‐effectiveness, scalability, high catalytic activity, and stability presents a significant challenge for zinc–air batteries (ZABs). The nitrogen‐rich lignin coordination network structure is synthesized through amine modification of lignin.
Ping‐Xian Feng +8 more
wiley +1 more source
通过8年田间定位试验,研究了不同施肥制度下褐土及其微团聚体有机碳活性变化规律。结果表明,褐土微团聚体有机碳活性随粒级的减小而增强,不同施肥制度下土壤微团聚体组成变化各异,不施肥主要是由于10 ...
韩志卿 +6 more
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