Results 241 to 250 of about 665,501 (321)

Workflow for Harmonic IR and Raman Spectra of Embedded Systems: The PE-QM Approach. [PDF]

open access: yesJ Phys Chem A
Vester J   +4 more
europepmc   +1 more source

Magnetic Field‐Driven Spin State Transformation in Promoting the Catalytic Activity of Doped Single‐Atom for Hydrogen Evolution Reaction

open access: yesAdvanced Materials, EarlyView.
A ferromagnetic RuSAs/Ni2P@Fe3O4 material is designed via a synergistic strategy of single‐atom doping and magnetic field‐driven spin‐state transformation. This strategy introduces new Ru single‐atom active sites for the hydrogen evolution reaction and facilitates the transition of Fe3+ (3d t2g) low‐spin electrons to a high‐spin state (3d eg ...
Chenjing Wang   +9 more
wiley   +1 more source

Active Learning‐Guided Accelerated Discovery of Ultra‐Efficient High‐Entropy Thermoelectrics

open access: yesAdvanced Materials, EarlyView.
An active learning framework is introduced for the accelerated discovery of high‐entropy chalcogenides with superior thermoelectric performance. Only 80 targeted syntheses, selected from 16206 possible combinations, led to three high‐performance compositions, demonstrating the remarkable efficiency of data‐driven guidance in experimental materials ...
Hanhwi Jang   +8 more
wiley   +1 more source

Stabilizing Frustrated Phase Transitions in Selective Oxidation Reactions

open access: yesAdvanced Materials, EarlyView.
Using multimodal operando spectromicroscopy, the frustrated phase transition responsible for selective oxidation over cobalt oxide spinel catalysts is identified, corresponding to combined surface reaction and Mars‐van Krevelen (MvK) dynamics. This regime is disrupted by the formation of mobile vacancies and the depletion of active oxygen at high ...
Luis Sandoval‐Diaz   +11 more
wiley   +1 more source

Macrophages Mediate Mesoscale Brain Mechanical Homeostasis

open access: yesAdvanced Materials, EarlyView.
We investigated the role of infiltrating immune cells in sculpting the developing brain. Using Brillouin microscopy and active microrheology, we found microglia actively maintain tissue viscoelasticity. Moreover, colony stimulating factor one receptor (CSF1R)‐driven stromal remodeling alters brain mechanics in vivo. These findings link immune activity,
Woong Young So   +11 more
wiley   +1 more source

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