Results 151 to 160 of about 32,444,034 (233)

Electrolyte–Framework Matching in High‐Voltage TEMPO‐COF Cathodes for Lithium Batteries

Advanced Science, EarlyView.
TEMPO‐functionalized covalent organic frameworks are investigated as high‐voltage cathodes for lithium batteries. Screening five electrolyte anions identifies lithium difluoro(oxalato)borate (LiDFOB) as the optimal electrolyte, balancing capacity, rate capability, and cycling stability, while buckypaper electrodes achieve high mass loading (40 mg cm−2)
Marilyn Esclance DMello, Nagaraj Patil, Fanni Fekecs, Sergio Pinilla, Rebeca Marcilla, Manuel Souto   +5 more
wiley   +1 more source

Recent Advances in Carbon Cathode Materials toward High‐Performing Zinc‐Ion Hybrid Supercapacitors

Advanced Science, EarlyView.
Aqueous zinc‐ion hybrid supercapacitors (ZHSCs) have emerged as promising next‐generation electrochemical energy‐storage devices. Porous carbon materials have been extensively studied as cathodes, with advances in tailoring pore structures and material properties to enhance performance.
Take Hirooka, Zhaolin Liu, Ivan P. Parkin, Guanjie He   +3 more
wiley   +1 more source

Automating Chemical Reasoning in High‐Throughput Phase Identification With a Probabilistic, LLM‐Guided Framework

Advanced Science, EarlyView.
Autonomous laboratories can now synthesize materials faster than experts can interpret the resulting diffraction data. A probabilistic framework combines refinement‐fit metrics with large language model‐derived chemical reasoning to rank competing phase interpretations and flag those unsuitable for autonomous use.
Olympia Dartsi, Lauren N. Walters, Amalie E. Trewartha, Steven B. Torrisi, Amanda Volk, Liam Joyce, Gerbrand Ceder, Anubhav Jain   +7 more
wiley   +1 more source

Physics‐Guided Descriptors Enable Data‐Efficient Prediction of Battery Coulombic Efficiency

Advanced Science, EarlyView.
This work integrates multiscale simulations with data‐driven approaches to predict Coulombic efficiency (CE). Multiscale simulations of battery systems are performed to extract Physics‐Guided descriptors and construct a dataset. Machine learning models trained on this dataset are then subjected to interpretable analysis to identify the most influential
Qintao Sun, Xuewei Gu, Yulin Jie, Hao Yang, Shuhong Jiao, Chao Tang, Yangping Sheng, Yuhao Lu, Ruiguo Cao, Tao Cheng   +9 more
wiley   +1 more source

Targeted Multifunctional Fluorine‐Rich Copolymer Coating Design for Ambient‐Stable Prelithiated SiOC Anodes

Advanced Science, EarlyView.
A fluorine‐rich acrylate copolymer, poly (tridecafluorooctyl methacrylate‐co‐methyl methacrylate) (PFMMA), is introduced as a multifunctional protective coating to stabilize the prelithiated SiOC electrodes in humid conditions and preserve unimpeded interfacial ion/charge transport during redox reactions.
Rong Chen, Yixuan Fan, Congcong Zhang, Yinan Liu, Yun Zheng, Ruifeng Zheng, Yingying Shen, Pingshan Jia, Luojiang Zhang, Yongbing Tang, Huaiyu Shao   +10 more
wiley   +1 more source

MgP4/CNT‐Graphene Embedded in Hard Carbon Matrix as a High‐Capacity Anode for Next‐Generation Sodium‐Ion Batteries

Advanced Science, EarlyView.
Phosphorus‐rich MgP4 is introduced as a high capacity anode for sodium‐ion batteries (SIBs) via hybrid carbon matrix engineering. A sequential CNT/G assembly forms a conductive and mechanically robust network, delivering a high reversible capacity of 1386 mAh g−1 while stabilizing alloying reactions.
Sion Ha, Doyeon Lee, Dong Won Kim, Won‐Sik Kim, Minkyu Lee, Seong‐Hyeon Hong, Kyeong‐Ho Kim   +6 more
wiley   +1 more source

In Situ Alkali Metal Exfoliation‐Coupled Dilute CO2 Electrolysis to Synthesize Interlayer‐Expanded Graphite for High‐Rate Lithium Storage

Advanced Science, EarlyView.
Converting CO2 into advanced carbon materials capable of meeting the rapid lithium storage demands of lithium‐ion batteries creates a mutually beneficial scenario for both energy and environmental sectors. Here, we propose a stepwise CO2 electrolysis approach to transform dilute CO2 into interlayer‐expanded graphite using molten salt electrolyzers ...
Hao Zha, Xiaodan Zhang, Xinyu Li, Jiajun Li, Yuxin Wu, Xiaoyang Wang, Huayi Yin, Dihua Wang, Bowen Deng   +8 more
wiley   +1 more source

Dynamic Interfacial pH Stabilization and (002) Oriented Deposition Enabled by Histidine‐Induced Solid Electrolyte Interphase for Highly Reversible Zn Anodes

Advanced Science, EarlyView.
The histidine‐induced ultrathin SEI (Zn(OH)2‐HIS) delivers exceptional anode stability by stabilizing the interfacial pH via a synergistic mechanism of chemical buffering and physical blocking, while inducing dendrite‐free oriented (002) deposition.
Qi Liu, Yimin Chen, Jianwei Lu, Xiangqun Zhuge, Xiyuan Zhong, Huaichong Sun, Yibing Li, Zhihong Luo, Kun Luo, Weiwei Lei, Dan Liu, Anjun Hu, Aijing Ma   +12 more
wiley   +1 more source

Unveiling Mechanisms of SEI Formation and Sodium Loss in Sodium Batteries via Interface Reactor Sampling

Advanced Science, EarlyView.
An “Interface Reactor” strategy boosts simulation stability by 2–3 orders of magnitude, enabling stable 100 ns molecular dynamics of electrode‐electrolyte interfaces. Distinct SEI formation mechanisms are revealed: mixed co‐formation in carbonates versus surface‐energy‐controlled NaF crystallization in ethers. Metadynamics simulations further elucidate
Zhoulin Liu, Ziliang Wang, Zherui Chen, Jianchun Sha, Fengzijun Pan, Pingyang Zhang, Yinghe Zhang   +6 more
wiley   +1 more source

In Situ Local Resistance Analysis of Mechanical Degradation in All‐Solid‐State Batteries

Advanced Science, EarlyView.
In this study, we developed an in situ scanning spreading resistance microscopy technique for all‐solid‐state batteries using sulfide solid electrolytes to visualize the evolution of local electronic resistance in NCM‐based cathode composites during charging.
Hirotada Gamo, Yasushi Maeda, Yuji Yamagishi, Tetsu Kiyobayashi, Naoya Ishida, Zyun Siroma, Kentaro Kuratani, Nobuhiko Takeichi, Hikaru Sano   +8 more
wiley   +1 more source