Results 71 to 80 of about 6,760,588 (269)

Ultrabroadband Excitation of Hot Carriers in Plasmonic Nanorods Revealed by Two‐Dimensional Electronic Spectroscopy

open access: yesAdvanced Optical Materials, EarlyView.
This work dissects the ultrafast response of polydisperse plasmonic nanorods using two‐dimensional electronic spectroscopy, uniquely combining temporal and spectral resolution. Our ultrabroadband pulses cover both transverse and longitudinal nanorods’ resonances, revealing sub‐200‐fs dynamics and distinct broadening mechanisms.
Andrea Schirato   +8 more
wiley   +1 more source

Unlocking Two‐Photon Chiral Signatures in DNA‐Stabilized Silver Nanoclusters: Two‐Photon Circular Dichroism and Circularly Polarized Luminescence

open access: yesAdvanced Optical Materials, EarlyView.
Chiroptical properties of DNA‐stabilized silver nanocluster (DNA)2​[Ag16​Cl2​]8+ are presented in linear and nonlinear regime. These water‐soluble, NIR‐emitting nanoprobes demonstrate exceptionally high two‐photon circular dichroism and circularly polarized luminescence brightness.
Karolina Sulowska   +3 more
wiley   +1 more source

Excitonic Landscapes in Monolayer Lateral Heterostructures Revealed by Unsupervised Machine Learning

open access: yesAdvanced Optical Materials, EarlyView.
Hyperspectral photoluminescence data from graded MoxW1 − xS2 alloys and monolayer MoS2–WS2 lateral heterostructures are analyzed using unsupervised machine learning. The combined use of PCA, t‐SNE, and DBSCAN uncovers distinct excitonic regions that trace how composition, strain, and defects modulate optical responses in these 2D materials.
Maninder Kaur   +4 more
wiley   +1 more source

Strong Proton‐Phonon Coupling Drives Fast Ion Transport in Perovskites

open access: yesAdvanced Science, EarlyView.
Experimental and computational phonon analysis of ABO3‐type proton conductor BaSnO3 shows that substitution on the B‐site with yttrium forms an imaginary phonon mode which is instrumental for the function as proton conductor. This overcompensates the adverse proton trapping effect of the yttrium.
Alexey Rulev   +8 more
wiley   +1 more source

Early Detection of Cell Death Using Transmembrane Water Exchange Magnetic Resonance Imaging

open access: yesAdvanced Science, EarlyView.
Cell death is important in both the development and treatment of cancer. In this study, it is demonstrated for the first time that a specific measurement of the transmembrane water exchange rate using magnetic resonance imaging can be used as an early marker of cell death in mammalian cells, in animals and in human patients. Abstract Cell death plays a
Athanasia Kaika   +22 more
wiley   +1 more source

Mapping Charge Interactions in Intrinsically Disordered Proteins

open access: yesAdvanced Science, EarlyView.
This study presents analytical models to predict intrachain distances in intrinsically disordered proteins (IDPs), accounting for charge patterning, salt concentration, and electrostatic effects. Validated against single‐molecule FRET data, a minimal‐parameter polymer model is identified that captures key interactions and chain dimensions. These models
Michael Phillips   +14 more
wiley   +1 more source

Ferromagnetic Interlayer Exchange Coupling in Magnetic Topological Insulator Sandwich Heterostructures

open access: yesAdvanced Science, EarlyView.
A thin topological insulator (Bi2Te3) inserted between two single magnetic septuple layers of MnBi2Te4 is shown to convert the intrinsic antiferromagnetic interlayer coupling into robust ferromagnetism. As the Bi2Te3 spacer thickness increases from 1 to 4 quintuple layers, the weakening coercivity, Curie temperature, and interlayer coupling reveal ...
Enayet Hossain   +10 more
wiley   +1 more source

Uncovering the Lipid Interface in Neurotransmission: Single Molecule Measurements of Neurotransmitters Interacting with Membranes Reveal Species Dependent Membrane Binding

open access: yesAdvanced Science, EarlyView.
Using single‐molecule whispering gallery mode sensors, neurotransmitter‐specific membrane binding signatures are measured that reveal intrinsically distinct interaction kinetics and orientations on a lipid membrane. Abstract Neurotransmitters (NTs) have traditionally been understood to act via aqueous‐phase receptor binding, but growing evidence ...
Thomas L. Derrien   +4 more
wiley   +1 more source

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