Results 141 to 150 of about 3,477,557 (293)

Modulation of Local Environment for Selective Bicarbonate Conversion to Multi‐Carbon Products

open access: yesAdvanced Energy Materials, EarlyView.
Highly porous Cu electrode partially coated with an ionomer/carbon composite enables efficient conversion of bicarbonate to multi‐carbon products. By regulating the local reaction microenvironment, this strategy overcomes selectivity and reaction‐rate limitations, achieving Faradaic efficiencies of 43% for ethylene and 60% for total multi‐carbon ...
Tai Nguyen   +15 more
wiley   +1 more source

Simultaneous Electronic and Crystallographic Modulation of Cs3Bi2Br9 by Single‐Element Sn Substitution for Enhanced CO2 Photoreduction

open access: yesAdvanced Energy Materials, EarlyView.
Aliovalent B‐site substitution with Sn2+ in lead‐free perovskite, Cs3Bi2Br9, is employed to simultaneously induce lattice contraction and bromine vacancy through charge imbalance and ionic radius mismatch. The resulting structural distortion modulates the electronic structure and improves charge separation, leading to enhanced visible‐light‐driven CO2 ...
Justin Khor   +7 more
wiley   +1 more source

Operando Identification of the Active Phase in Sr‐Promoted Lanthanum Cobaltite Perovskite‐Derived Catalysts for Ammonia Decomposition

open access: yesAngewandte Chemie, EarlyView.
Ammonia decomposition catalyzed by base metals: Exsolution of cobalt from perovskites prepared by spray‐flame synthesis (SFS) yields highly active, SrO‐promoted Co/La2O3 catalysts with low cobalt content. Operando studies provide insight into the function of the promoter. Dynamic surface reconstruction under operating conditions increases the interface
Barış Alkan   +16 more
wiley   +2 more sources

Role of buoyant flame dynamics in wildfire spread. [PDF]

open access: yesProc Natl Acad Sci U S A, 2015
Finney MA   +9 more
europepmc   +1 more source

Breaking the Polarity–Coordination Coupling in Electrolyte Design for High‐Voltage Lithium Batteries

open access: yesAdvanced Energy Materials, EarlyView.
Steric and electronic co‐regulation of 2,2,2‐trifluoro‐N, N‐dimethylethylamide (DMTFA) decouples high polarity from strong Li+ coordination, creating an anion‐mediated pseudo‐weakly solvating electrolyte. This design lowers Li+ desolvation barriers, enhances Li+ mobility, and builds B‐, F‐, and N‐rich inorganic interphases, enabling stable 3.0–4.6 V ...
Xue Li   +9 more
wiley   +1 more source

Multifunctional Matrix‐Activated Electrodes Enabling Efficient Proton Transport and Durable Low‐Pt Operation for High‐Temperature Proton Exchange Membrane Fuel Cells

open access: yesAdvanced Energy Materials, EarlyView.
This work introduces a CeHP‐enabled multifunctional matrix‐activated electrode (MME) for high‐temperature PEM fuel cells, forming an electrochemically and mechanically functional matrix within the catalyst layer. The design increases peak power density by 38% and reduces voltage decay by 62% at 240 °C, while using only 40% of the Pt loading of a ...
Gyeongseok Gwak   +12 more
wiley   +1 more source

Synthesis of Ladder and Flexible Polysulfonimides Directly From Anionic Monomers: Investigating Structure–Property Convergence in Succinonitrile–Polymer Electrolyte Blends

open access: yesAngewandte Chemie, EarlyView.
Direct synthesis of sulfonimide‐based polymers of intrinsic microporosity enables comparison with compositionally similar flexible analogs. Incorporation of a common pore‐filling transport medium drives these fundamentally different polymer architectures toward similar bulk conductivity and mechanical properties while revealing distinct microscopic ion‐
Abraham Herzog‐Arbeitman   +8 more
wiley   +2 more sources

Competing Charge Separation Pathways Govern Charge Generation in Organic Photovoltaic Blends: Insights From Transient Electron Spin Resonance

open access: yesAdvanced Energy Materials, EarlyView.
Transient electron spin resonance distinguishes interfacial charge‐transfer states from separated charges, revealing competing charge separation pathways in organic photovoltaic blends. The relative contributions of fast charge separation and a pathway mediated by spin‐polarized charge‐transfer states vary across different blends, with high‐efficiency ...
Jack M. S. Palmer, Claudia E. Tait
wiley   +1 more source

Flame dynamics of a meso-scale heat recirculating combustor

open access: yes
The dynamics of premixed propane-air flame in a meso-scale ceramic combustor has been examined here. The flame characteristics in the combustor were examined by measuring the acoustic emissions and preheat temperatures together with high-speed ...
Gupta, A.K., Vijayan, V.
core  

Surface‐Functionalized MXene for Enhanced Photocatalytic CO2 Reduction

open access: yesAdvanced Energy Materials, EarlyView.
Poly(catechol/p‐cresol)‐functionalized MXene (f‐MXene) enhances oxidation stability while preserving conductivity, enabling efficient interfacial electron transfer in a Cu/f‐MXene/reduced TiO2 photocatalyst. Strong Cu–f‐MXene synergy promotes CO2 activation and selective CH4 production, achieving a CH4 yield of 18.1 µmol g−1 (>200 × vs.
Dongyun Kim   +18 more
wiley   +1 more source

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