Results 191 to 200 of about 1,526,395 (305)

Engineering Relative Spatial Structure of Dual Atomic Sites with Asymmetric Coordination for High‐Performance Hydrogen Evolution Activity

open access: yesAdvanced Functional Materials, EarlyView.
Dual‐atom catalysts featuring varying spatial configurations of metal sites (Pt1Fe1 DACs) are employed to systematically investigate the influence of spatial arrangements on the electronic structure and catalytic activity of active sites. Notably, the 3D asymmetric Pt1Fe1‐TAC dimer, featuring strong interatomic interactions, demonstrates superior ...
Yi Guan   +8 more
wiley   +1 more source

Atomic‐Level Dual‐Cation Engineering Enables High‐Performance Na4VMn(PO4)3 Cathodes for Sodium‐Ion Batteries

open access: yesAdvanced Functional Materials, EarlyView.
Dual‐cation site engineering unlocks stable and fast sodium storage in Na4VMn(PO4)3 cathodes. Li+ at Na2 suppresses Jahn‐Teller distortion, while K+ at Na1 expands ion channels, enabling synchronized V/Mn redox and quasi‐single‐phase kinetics. This atomic‐level strategy achieves ultralong cycling stability, high‐rate capability, and full cell viability
Jiaze Sun   +8 more
wiley   +1 more source

Biomimetic Ion‐Orchestrated Hierarchical Armored Hydrogel Coating for Robust and Multifunctional Surface Protection

open access: yesAdvanced Functional Materials, EarlyView.
Inspired by the skin‐toughening mechanism of marine sponges, an ion‐orchestrated structural engineering strategy is proposed to regulate the surface microstructure of hydrogel coatings, enabling the in situ formation of a robust armor layer that enhances mechanical integrity and provides multifunctional protection by suppressing fouling attachment and ...
Wenshuai Yang   +11 more
wiley   +1 more source

Enhanced Nitric Oxide Electroreduction to Ammonia via Modulating Spin‐Polarization of Fe Single‐Atom Catalysts

open access: yesAdvanced Functional Materials, EarlyView.
A strategic spin‐polarization suppression in Fe single‐atom catalysts is proposed to enhance electrocatalytic reduction of NO to NH3. Employing a top‐down electrospinning strategy, self‐supported FeSAC with Fe‐N3S1 coordination structure and spin‐state transition is engineered from high‐spin to low‐spin.
Jialing Song   +13 more
wiley   +1 more source

Artificial Amorphous Interface Matters for Boosting High‐Voltage Stable LiCoO2 Cathode

open access: yesAdvanced Functional Materials, EarlyView.
The amorphization of phosphate‐based surface layer with favorable Li‐ion conducting kinetics is realized by precisely tailored atomic‐level fabrication. This amorphous coating enables the lithium cobalt oxide (LCO) cathode superior high‐voltage rate capability and cycling performance, owing to the fast interfacial ionic transport and maintained ...
Jinjin Ma   +10 more
wiley   +1 more source

Fluoride‐Free Adhesives for Low Surface Energy Fluorinated Substrates

open access: yesAdvanced Functional Materials, EarlyView.
A universal, fluoride‐free adhesive achieves a record 4.91 MPa bond strength on PTFE by leveraging amine/amide dipole–dipole interactions, without fluorinated components. This sustainable strategy overcomes the environmental and performance limits of PFAS‐based adhesives, enabling robust, eco‐conscious bonding across diverse materials.
Siqi Zheng   +7 more
wiley   +1 more source

Geometrically‐Screened, Sterically‐Hindered Additive for Wide‐Temperature Aqueous Zinc‐Ion Batteries

open access: yesAdvanced Functional Materials, EarlyView.
A molecular‑engineering strategy combining steric hindrance tuning with geometric optimization identifies cellobiose as an ideal additive for aqueous zinc‑ion batteries, enabling stable Zn deposition across a wide temperature range from −30 to 50 °C. Abstract Aqueous zinc‐ion batteries (AZIBs) are emerging as a highly promising alternative to lithium ...
Sida Zhang   +13 more
wiley   +1 more source

Switchable Supramolecular Adhesive by Tuning Interfacial Bonding and Modulus

open access: yesAdvanced Functional Materials, EarlyView.
The supramolecular adhesive (HyDiP) shows reversible adhesion and recyclability. In the dehydrated state, it is dense, stiff (E ≈445 MPa), transparent, and provides strong bonding with adhesion strengths up to 4.65 MPa. In the hydrated state, it becomes porous, soft (E ≈0.11 MPa), and detaches easily, enabling sustainable high‐strength applications ...
Rumin Fu   +10 more
wiley   +1 more source

Photothermal Macroporous Lignin Cryogels for Off‐Grid, Continuous Atmospheric Water Collection via Interlayer Heat Recovery

open access: yesAdvanced Functional Materials, EarlyView.
Photothermal, macroporous lignin‐based cryogels are engineered to convert sunlight into low‐grade heat. Integrated as stacked beds in a drum‐type device, a thin copper interlayer transfers waste heat between beds, enabling interlayer heat recovery and continuous solar cycling.
Jie Yan   +8 more
wiley   +1 more source

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