Results 111 to 120 of about 181,157 (281)

On the Role of Reaction Current Distribution to Attain Competitive Solid‐State Batteries

Angewandte Chemie, EarlyView.
We conducted a case study on reaction current inhomogeneities when increasing areal loadings and charging rates in NCM‐argyrodite composite cathodes for solid‐state batteries. Using a combination of cycling experiments and operando high‐energy X‐ray diffraction, we show that employing faster conducting Li5.5PS4.5Cl1.5 instead of Li6PS5Cl as catholyte ...
Johannes Hartel, Lukas Ketter, Eva Schlautmann, Erik Šimon, Karol Végsö, Poongodi Ayyanusamy, Tim Bernges, Peter Siffalovic, Wolfgang G. Zeier   +8 more
wiley   +2 more sources

A Concept for a Multipurpose Time-of-Flight Neutron Reflectometer at Compact Neutron Sources

Instruments
The design of a time-of-flight neutron reflectometer proposed for the new generation of compact neutron sources is presented. The reflectometer offers the possibility to use spin-polarized neutrons. The reflectometer design presented here takes advantage
Raul-Victor Erhan, Victor-Otto de Haan, Christoph Frommen, Kenneth Dahl Knudsen, Isabel Llamas-Jansa, Bjørn Christian Hauback   +5 more
doaj   +1 more source

Disorder‐Driven Fast Na+ Transport: From Crystalline to Amorphous Networks in the Mixed‐Anion NaTaOxCl6−2x Oxychlorides

Advanced Energy Materials, EarlyView.
Oxygen substitution in NaTaOxCl6‐2x drives structural evolution from isolated [TaCl6]– octahedra, through oxygen‐bridged [Ta2OCl10]2– dimers, toward extended trans‐[TaO2Cl4]3– chain‐like arrangements. At intermediate compositions, zero‐dimensional corner‐sharing motifs are proposed to create a flexible, disordered framework that peaks ionic ...
Justin Leifeld, Abigail C. Parsons, Alexandra Morscher, Xabier Martinez de Irujo‐Labalde, Marvin A. Kraft, Oskar G. Soulas, Bibek Samanta, Wiebke Zielasko, Neelam Yadav, Kyra Strotmann, Niina Jalarvo, Bruno V. M. Rodrigues, Adam Slabon, Philipp Adelhelm, Michael Ryan Hansen, David O. Scanlon, Wolfgang G. Zeier, Alexander G. Squires   +17 more
wiley   +1 more source

Machine-Learning-Based Real-Time, High-Fidelity Neutron Source Identification via Cavitation Acoustic Shock Spectra in Centrifugally Tensioned Metastable Fluid Detectors

IEEE Access
Neutron source spectrometry and energy discrimination represent a time-consuming, laborious endeavor requiring complex instrumentation across the nuclear science and technology sector affecting diverse fields such as nuclear power, radiation safety ...
Bailey Christensen, Rusi Taleyarkhan
doaj   +1 more source

A Quantitative Lithium Inventory Framework for Anode‐Free Lithium Metal Batteries

Advanced Energy Materials, EarlyView.
A component‐resolved lithium inventory framework quantitatively tracks Li redistribution across the cell in anode‐free NMC622||Cu pouch cells throughout cycling. Three sequential degradation stages are identified: formation‐driven cathode Li depletion, midlife inactive Li0 accumulation, and late‐stage runaway SEI thickening. The cathode, as the sole Li
Wurigumula Bao, Alex Liu, Thomas S. Marchese, Yuanlong Bill Zheng, Weikang Li, Dhevathi Rajan Rajagopalan Kannan, Vallabha Rao Rikka, Vinay Premnath, Judith Jeevarajan, Ying Shirley Meng   +9 more
wiley   +1 more source

Hydrogels Under Superchaotropic Control: Polyoxometalate Stabilization and pH‐Responsive Crosslinking in Cellulose Ether Solutions

Angewandte Chemie, EarlyView.
Superchaotropic binding of Keggin polyoxometalates (POMs) to non‐ionic biopolymers like cellulose ethers (CEs) stabilizes otherwise hydrolytically unstable POMs in aqueous solution and allows conversion of pH‐nonresponsive polymers into pH‐responsive soft materials. The pH‐driven conversion from plenary to lacunary POMs switches superchaotropic binding
Vighnesh B. Lokare, Amina Ledinic, Nina Wehr, Max Hohenschutz   +3 more
wiley   +2 more sources

Comparison of DeePMD, MTP, GAP, ACE and MACE Machine‐Learned Potentials for Radiation‐Damage Simulations: A User Perspective

Advanced Intelligent Discovery, EarlyView.
The authors evaluated six machine‐learned interatomic potentials for simulating threshold displacement energies and tritium diffusion in LiAlO2 essential for tritium production. Trained on the same density functional theory data and benchmarked against traditional models for accuracy, stability, displacement energies, and cost, Moment Tensor Potential ...
Ankit Roy, Ram Devanathan, Sarah Allec, Giridhar Nandipati, Andrew M. Casella, David J. Senor, Duane D. Johnson, Ganesh Balasubramanian, Ayoub Soulami   +8 more
wiley   +1 more source

Site‐Selective B─H Activation via HAT Toward Xanthyl‐closo‐Carboranes as Bench‐Stable Precursors of Organosulfur Boron Clusters

Angewandte Chemie, EarlyView.
A light mediated direct regioselective B─H functionalization, via hydrogen atom transfer (HAT), is described. Unexplored xanthyl‐closo‐carboranes as novel bench‐stable and versatile platforms to access sulfur‐containing boron clusters are reported for the first time.
Marco Rusconi, Eugenia Magi, Polyssena Renzi, Emanuele Azzi, Valeria Lagostina, Enrico Salvadori, Mario Chiesa, Birgit Hischa, Giovanni Ghigo, Annamaria Deagostino   +9 more
wiley   +2 more sources

Optimizing neutron shielding: A specialised container approach for Disused Sealed Radioactive Sources and orphan neutron emitters

Nuclear Analysis
Shielding Disused Sealed Radioactive Sources (DSRSs) and orphan neutron sources, such as 252Cf, pose challenges due to the high penetration of neutrons, induced radioactivity in shielding materials, and the limited availability of compact, effective ...
Brahim EL Azzaoui, Ouadie Kabach, Mohamed Youssef Messous, El mahjoub Chakir, El Mehdi Alibrahmi   +4 more
doaj   +1 more source

Autonomous AI‐Driven Design for Skin Product Formulations

Advanced Intelligent Discovery, EarlyView.
This review presents a comprehensive closed‐loop framework for autonomous skin product formulation design. By integrating artificial intelligence‐driven experiment selection with automated multi‐tiered assays, the approach shifts development from trial‐and‐error to intelligent optimisation.
Yu Zhang, Yongrui Xiao, Chunlin Chen, Dimitrios Tsaoulidis, Kai Yang, Tao Chen   +5 more
wiley   +1 more source