Results 51 to 60 of about 26,915 (263)

Mechanistic Control of C─H Bond Activation and C─C Coupling in Light‐Driven Methane Conversion to C2+ Products over Multifunctional Photocatalysts

Advanced Functional Materials, EarlyView.
Methane photocatalytic activation under mild conditions remains a formidable challenge in the synthesis of solar fuels. In this review, we emphasize the growing importance of multifunctional materials and hybrid systems within a unified mechanistic framework that integrates selective C─H bond activation, formation and control of intermediates, C─C ...
Di Hu, Yuheng Jiang, Vitaly V. Ordomsky, Bastian Mei, Zhiyong Tang, Andrei Y. Khodakov   +5 more
wiley   +1 more source

An Organic Borate Salt with Superior p‐Doping Capability for Organic Semiconductors

Advanced Science, 2020
Molecular doping allows enhancement and precise control of electrical properties of organic semiconductors, and is thus of central technological relevance for organic (opto‐) electronics.
Berthold Wegner, Dominique Lungwitz, Ahmed E. Mansour, Claudia E. Tait, Naoki Tanaka, Tianshu Zhai, Steffen Duhm, Michael Forster, Jan Behrends, Yoshiaki Shoji, Andreas Opitz, Ullrich Scherf, Emil J. W. List‐Kratochvil, Takanori Fukushima, Norbert Koch   +14 more
doaj   +1 more source

Polarization‐Dependent Synaptic‐Like Electro‐Optical Response in Ferroelectric Nematic Liquid Crystals

Advanced Functional Materials, EarlyView.
Ferroelectric nematic liquid crystals (FNLCs) offer fast, tunable polarization and low‐voltage operation but suffer from poor polarization retention at zero field. Semiconductor‐modified FNLCs enhance polarization retention and exhibit short‐ and long‐term electro‐optical responses, while also supporting spike‐type signal integrations.
Kutay Sagdic, Weiming Yao, Danqing Liu
wiley   +1 more source

Bio‐Derived Polyelectrolyte Additive–Induced Interfacial Ion‐Diffusion Barriers for Nonvolatile Organic Artificial Synapses

Advanced Functional Materials, EarlyView.
Sodium alginate regulates interfacial ion transport and retention in electrolyte‐gated synaptic transistors. The carboxylate‐rich polymeric network forms a dynamic interfacial ion‐diffusion barrier that facilitates ion injection during programming while suppressing ion back‐diffusion, thereby stabilizing the electrochemically doped channel state.
Chaeyeon Han, Donghwa Lee, Hyeonse Kim, Hyoik Jang, Sein Chung, Geun Yeol Bae, Eunho Lee   +6 more
wiley   +1 more source

Charge Generation and Recombination Pathways in All‐Polymer Bulk Heterojunction Solar Cells

Advanced Functional Materials, EarlyView.
Multimodal spectroscopy and device analysis reveal how field‐dependent charge generation, transport limitations, and non‐geminate recombination govern performance losses in all polymer solar cells. The results identify the key processes controlling charge extraction and recombination, providing insights for the design of more efficient all‐polymer ...
Shahidul Alam, Wejdan Althobaiti, Safakath Karuthedath, Christopher E. Petoukhoff, Amr Dahman, Khawla Alkhezaim, Oleksandr Matiash, José P. Jurado, Mariia Ferree, Ning Su, Jacob Blaskovits, Denis Andrienko, Vladimir Dyakonov, Andreas Sperlich, Vojtech Nádaždy, Tobin J. Marks, Antonio Facchetti, Frédéric Laquai   +17 more
wiley   +1 more source

Si‐Doped Nanocrystalline Diamond as Highly Sensitive Luminescence Thermometer for the Physiological Temperature Range

Advanced Functional Materials, EarlyView.
In this work, diamonds with negative charged silicon‐vacancy (SiV−) centers have been designed for use as thermometers in biomedical applications. Multiparametric analysis of the emission characteristics of the SiV− centers provides extraordinary sensitivity for temperature detection in the physiological temperature range.
María Gragera, Iván Carrillo‐Berdugo, Josue Millán, Paulius Pobedinskas, Antonio Freire, Ken Haenen, Javier Navas   +6 more
wiley   +1 more source

High‐Performance n‐Type Organic Thermoelectrics Enabled by Control Over Microstructure, Orientation and Contact Plane in Naphthalenediimide‐Bithiazole‐Copolymer Films

Advanced Functional Materials, EarlyView.
Effective control over the crystalline contact plane and microstructure of a naphthalenediimide‐bithiazole copolymer enables high‐performance n‐type thermoelectrics. While rubbing alignment induces a detrimental edge‐on orientation, subsequent solvent vapor‐induced re‐orientation facilitates a favorable mixed face‐on/edge‐on morphology.
Suhao Wang, Said Oummouch, Huan Wei, Karl Thorley, Adam Marks, Arianna Magni, Xiuming Sun, Alessandra Pistillo, Bruno Schmaltz, Olivier Bardagot, Sabine Ludwigs, Alberto Salleo, Yuanyuan Hu, Martin Brinkmann   +13 more
wiley   +1 more source

Strong Acceptors Based on Derivatives of Benzothiadiazoloimidazole

Molecules
Despite the rapid progression of organic semiconductors, developing high-air-stability n-type organic semiconductors are still challenging. Herein, novel strong acceptors based on benzothiadiazoloimidazole units are reported.
Hanyun Du, Bin Chen, Fengyuan Zhang
doaj   +1 more source

Bismuth‐Based Photocatalysts for Water Remediation: Design Strategies, Mechanisms, and Challenges

Advanced Functional Materials, EarlyView.
This review highlights representative design strategies for bismuth‐based semiconductor photocatalysts in solar‐driven water purification. Emphasis is placed on electronic structure regulation, oxygen‐vacancy engineering, and interfacial coupling to enable efficient full‐spectrum light utilization, improved charge separation, and selective oxidation in
Shan Liu, Yi Zhao, Liming Cai, Simin Long, Jing Kang, Jingkai Lin, Jimin Shen, Zhonglin Chen, Shaobin Wang, Huayang Zhang   +9 more
wiley   +1 more source

Angle-Resolved Photoemission Study on the Band Structure of Organic Single Crystals

Crystals, 2020
Angle-resolved photoemission spectroscopy (ARPES) is a vital technique, collecting data from both the energy and momentum of photoemitted electrons, and is indispensable for investigating the electronic band structure of solids.
Ke Wang, Ben Ecker, Yongli Gao
doaj   +1 more source