Results 261 to 270 of about 1,453,193 (347)

New proton emitter <sup>188</sup>At implies an interaction unprecedented in heavy nuclei. [PDF]

open access: yesNat Commun
Kokkonen H   +23 more
europepmc   +1 more source

Covalent Adaptable Networks with Associative Siloxane Exchange Enabled by Amide‐Based Internal Catalysis: Designing for Reprocessability and Extrudability by Increasing the Cross‐Link Density

open access: yesAdvanced Functional Materials, EarlyView.
Internally catalyzed siloxane dynamic chemistry is demonstrated resulting from amides covalently linked through alkyl chains to siloxanes. The alkyl length in the siloxane‐containing monomer tunes the network cross‐link density. Siloxane exchange dynamics are faster with increasing cross‐link density, because associative exchange is second order in ...
Nathan S. Purwanto   +5 more
wiley   +1 more source

Highly Sensitive Electrochemical Biosensor Based on Hairy Particles with Controllable High Enzyme Loading and Activity

open access: yesAdvanced Functional Materials, EarlyView.
For the first time, a highly sensitive electrochemical biosensor based on SiO2‐based hairy particles with a grafted PDMAEMA polymer brush containing a quantifiable and large amount of immobilized Laccase is reported. The fabricated biosensor exhibits a sensitivity of 0.14 A·m⁻¹, a limit of detection (LOD) of 0.1 µm, and a detection range of 0.3–750 µm,
Pavel Milkin   +7 more
wiley   +1 more source

Fine‐Tunning BaCo0.4Fe0.4Zr0.1Y0.1O3−δ‐Based Air Electrodes for Reversible Protonic Ceramic Cells via Co‐Engineering A‐site Deficiency and Nickel Content

open access: yesAdvanced Functional Materials, EarlyView.
A synergistic strategy combining A‐site deficiency and B‐site nickel doping yielded a BCFZYN‐095‐01 nanocomposite air electrode for reversible protonic ceramic cells with superior ORR/OER activities. B‐site deficiency in the perovskite lattice enhances proton conduction, and nickel doping within the bulk facilitates oxygen transport.
Mingzhuang Liang   +12 more
wiley   +1 more source

Photocatalytic Versus Stoichiometric Hydrogen Generation Using Mesoporous Silicon Catalysts: The Complex Role of Sacrificial Reagents

open access: yesAdvanced Functional Materials, EarlyView.
This study highlights the importance of accounting for stoichiometric hydrogen produced when utilizing Si photocatalysts. The stoichiometric contribution is sacrificial reagent dependent and decreases with increasing sterics around the catalyst surface.
Sarrah H. Putwa   +4 more
wiley   +1 more source

Advancing the Co‐Based Anode Catalysts Using Ionomers in Pure‐Water Anion Exchange Membrane Electrolyzers

open access: yesAdvanced Functional Materials, EarlyView.
The role of ionomers is investigated in advancing cobalt‐based oxygen evolution catalysts in pure‐water anion exchange membrane electrolysers. Using in situ electrochemical analysis, ex situ material characterization, and membrane potential sensing, it is observed surface reconstruction at high currents and mitigated it via ionomer coating, achieving ...
Sanghwi Han   +6 more
wiley   +1 more source

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