Results 71 to 80 of about 1,288 (197)

Vibrational Circular Dichroism Spectra of 2,5‐Diaminoterephtalate Macrocycles Reveal Distant Vibrational Exciton Coupling

open access: yesChemistry – A European Journal, EarlyView.
The energy level diagrams for the ν(C═O) and the δ(N─H) vibrations, resulting of combining in‐phase and out‐of‐phase modes on the basis of their local symmetries, was built by applying the exciton coupling theory to a new class of chiral macrocycles, based on the 2,5‐diaminoterephthalate scaffold.
Samara Medina   +4 more
wiley   +1 more source

Quantifying Quantumness of Channels Without Entanglement

open access: yesPRX Quantum, 2022
Quantum channels breaking entanglement, incompatibility, or nonlocality are defined as such because they are not useful for entanglement-based, one-sided device-independent, or device-independent quantum-information processing, respectively.
Huan-Yu Ku   +10 more
doaj   +1 more source

Nitrogen‐Site Isomerism Unlocks Exciton Dissociation in Vinylene‐Linked COF‐Based Photocatalysts

open access: yesEcoEnergy, EarlyView.
Two regioisomeric vinylene‐linked covalent organic frameworks (COFs) constructed from diazine units with different nitrogen positions are developed for photocatalytic hydrogen evolution reaction (HER). Although structurally similar, the isomeric COFs exhibit distinct electron distribution and charge‐separation behaviors, leading to a more than twofold ...
Ming Wang   +10 more
wiley   +1 more source

Connector Tensor Networks: A Renormalization-Type Approach to Quantum Certification

open access: yesPhysical Review X, 2020
As quantum technologies develop, we acquire control of an ever-growing number of quantum systems. Unfortunately, current tools to detect relevant quantum properties of quantum states, such as entanglement and Bell nonlocality, suffer from severe ...
Miguel Navascués   +2 more
doaj   +1 more source

Confined Hot Carrier Cooling Via Excited‐State Energy Gap Engineering in Graphyne Carbon Allotropes

open access: yesENERGY &ENVIRONMENTAL MATERIALS, EarlyView.
The excited‐state energy gap (EEG), regulated by the concentration of sp‐hybridized carbon, provides an effective handle for tuning electron–phonon coupling behavior. This design enables long‐lived confinement of hot carriers near the top of the EEG with controllable energy levels.
Fulong Dai   +9 more
wiley   +1 more source

Nonlocality of quantum states can be transitive

open access: yesnpj Quantum Information
Despite the monogamous nature of nonlocal correlations, in a Bell test involving three parties A, B, and C, the nonlocality in two bipartite subsystems (e.g., AB and BC) may force the remaining bipartite subsystem (e.g., AC) to exhibit nonlocality ...
Kai-Siang Chen   +4 more
doaj   +1 more source

Low‐Dimensional Materials and Van Der Waals Heterostructures for Energy Application: A Comprehensive Review

open access: yesENERGY &ENVIRONMENTAL MATERIALS, EarlyView.
Low‐dimensional materials (0D, 1D, and 2D) exhibit unique electronic and physicochemical properties, enabling advanced nanoelectronic and optoelectronic devices. Mixed‐dimensional heterostructures combine these materials to enhance functionality.
Qaisar Alam   +3 more
wiley   +1 more source

Stimulated Forward Brillouin Scattering in Subwavelength Grating Silicon Membranes

open access: yesLaser &Photonics Reviews, EarlyView.
This work proposes a novel strategy to achieve large Brillouin scattering with independent control of the optical and mechanical modes using subwavelength silicon membranes. We experimentally demonstrate remarkably high Brillouin gain, resulting in an on/off Stokes gain of 3 dB and anti‐Stokes loss of 4 dB in a 6 mm‐long waveguide with 35 mW of on‐chip
Paula Nuño Ruano   +8 more
wiley   +1 more source

Quantization of Polaritons Confined in Dielectric Structures

open access: yesLaser &Photonics Reviews, EarlyView.
This study addresses the limitations of the Hopfield model of strong light‐matter coupling in the case of structured dieletrics. A method to derive quantum models in the polariton basis using Bogoliubov transformation and third quantization is introduced, demonstrating how to boost interaction strength and engineer nonlocal interactions for strongly ...
Amir Rahmani   +4 more
wiley   +1 more source

Spatial Orientation‐Dependent Double Hydrogen Bond/Photoredox Cooperative Catalysis in Metal–Organic Frameworks

open access: yesAngewandte Chemie, Volume 138, Issue 32, 3 August 2026.
We report a heterogeneous double hydrogen bond/photoredox synergistic catalysis, wherein the flexibility and spatial orientation of catalytic centers, rather than catalyst activity, play a dominant role in catalytic performance. ABSTRACT Catalyst activity is typically the primary priority in designing a catalytic system. The higher catalyst activity is
Jing Ouyang   +8 more
wiley   +2 more sources

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