A Quantitative Lithium Inventory Framework for Anode‐Free Lithium Metal Batteries
A component‐resolved lithium inventory framework quantitatively tracks Li redistribution across the cell in anode‐free NMC622||Cu pouch cells throughout cycling. Three sequential degradation stages are identified: formation‐driven cathode Li depletion, midlife inactive Li0 accumulation, and late‐stage runaway SEI thickening. The cathode, as the sole Li
Wurigumula Bao +9 more
wiley +1 more source
Revealing the roles of the solid-electrolyte interphase in designing stable, fast-charging, low-temperature Li-ion batteries. [PDF]
Tao L +18 more
europepmc +1 more source
Reliable Evaluation of Na‐Ion Battery Materials: Eliminating Na‐Metal Distortions
Na metal is highly reactive in carbonate electrolytes, forming unstable interphases and triggering parasitic reactions that distort measurements and undermine reproducibility. To enable accurate evaluation of materials for Na‑ion batteries, this work suggests that NASICON‑type counter electrodes provide a practical and stable platform for distortion ...
Jinkwang Hwang +9 more
wiley +1 more source
An in-depth Study of the Solid Electrolyte Interphase Compositional Evolution in Sodium-Ion Batteries: Unravelling the Effects of a Na Metal Counter Electrode on the SEI. [PDF]
Fitzpatrick JR +7 more
europepmc +1 more source
Machine learning interatomic potentials bridge quantum accuracy and computational efficiency for materials discovery. Architectures from Gaussian process regression to equivariant graph neural networks, training strategies including active learning and foundation models, and applications in solid‐state electrolytes, batteries, electrocatalysts ...
In Kee Park +19 more
wiley +1 more source
Tracking dendrites and solid electrolyte interphase formation with dynamic nuclear polarization-NMR spectroscopy. [PDF]
Maity A +4 more
europepmc +1 more source
Silicon anodes in sulfide SSBs face coupled electrochemo‐mechanical failure by interface instability. This review examined recent advances and proposed mitigation strategies via material‐, electrode/interface‐, and cell‐level‐ engineering. We further evaluate scalable synthesis of sulfide SEs.
Murugesan Karuppaiah +4 more
wiley +1 more source
Li<sub>7</sub>La<sub>3</sub>Zr<sub>2</sub>O<sub>12</sub>/Polymethacrylate-Based Composite Electrolyte with Hybrid Solid Electrolyte Interphase for Ultra-stable Solid-State Lithium Batteries. [PDF]
Li T +7 more
europepmc +1 more source
In Situ Evolution of Artificial Interphase Enabling Stable, High‐Performance Lithium Metal Batteries
An evolutionary artificial interphase is presented for stable lithium metal batteries. A Mg3N2‐based layer spontaneously evolves into a hybrid interphase enriched with superionic Li3N and lithiophilic Mg‐Li alloy during cycling. This dynamic, self‐reinforcing mechanism effectively suppresses dendrite growth and enables exceptional long‐term cycling ...
Sangcheol Lee +4 more
wiley +1 more source
Superior High-Rate Ni-Rich Lithium Batteries Based on Fast Ion-Desolvation and Stable Solid-Electrolyte Interphase. [PDF]
Xiao Z +6 more
europepmc +1 more source

