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Chemical Communications, 2021
A water-soluble and air-stable thermally activated delayed fluorescence (TADF) emitter was prepared by a nanoencapsulation strategy, which enables electrochemiluminescence (ECL) of TADF emitters in aqueous media for the first time.
Zihui Zeng +9 more
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A water-soluble and air-stable thermally activated delayed fluorescence (TADF) emitter was prepared by a nanoencapsulation strategy, which enables electrochemiluminescence (ECL) of TADF emitters in aqueous media for the first time.
Zihui Zeng +9 more
openaire +2 more sources
The Journal of Physical Chemistry Letters, 2022
Organic light-emitting diodes (OLEDs) still face a significant challenge in finding blue thermally activated delayed fluorescence (TADF) emitters that can achieve narrowband emission and high efficiency. In this work, we successfully design and synthesize a novel kind of TADF emitters based on rigid sulfur/oxygen-bridged triarylboron acceptor for ...
Honglei Gao +9 more
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Organic light-emitting diodes (OLEDs) still face a significant challenge in finding blue thermally activated delayed fluorescence (TADF) emitters that can achieve narrowband emission and high efficiency. In this work, we successfully design and synthesize a novel kind of TADF emitters based on rigid sulfur/oxygen-bridged triarylboron acceptor for ...
Honglei Gao +9 more
openaire +2 more sources
Donor-spiro-acceptor architecture for green thermally activated delayed fluorescence (TADF) emitter
Organic Electronics, 2020Abstract The rational molecular modification is an attractive area of interest to design new materials having promising results in organic light emitting diodes (OLEDs). Herein, a new green thermally activated delayed fluorescence (TADF) emitter, 2,7-bis(dimesitylboranyl)-9′,9′-dimethyl-9′H-spiro[fluorene-9,5′-quinolino[3,2,1-de]acridine] (ACS-BM ...
Aziz Khan +6 more
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Acta Crystallographica Section C Structural Chemistry, 2019
4,4′-{9,9′-Spirobi[10H-acridine]-10,10′-diyl}dibenzoic acid (L, C29H26N2O4) was designed and synthesized as a new donor–acceptor motif molecule. Due to the large dihedral angle between the planes of the carboxyphenyl group and the spiroacridine moiety, L possess thermally activated delayed fluorescence (TADF).
Xiu-Hui Ren +5 more
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4,4′-{9,9′-Spirobi[10H-acridine]-10,10′-diyl}dibenzoic acid (L, C29H26N2O4) was designed and synthesized as a new donor–acceptor motif molecule. Due to the large dihedral angle between the planes of the carboxyphenyl group and the spiroacridine moiety, L possess thermally activated delayed fluorescence (TADF).
Xiu-Hui Ren +5 more
openaire +2 more sources
The Journal of Physical Chemistry C, 2016
The increasing demand for high-performance organic light-emitting devices (OLEDs) based on thermally-activated delayed fluorescence (TADF) principle urgently requires to establish an efficient preparation strategy of high-performance TADF materials. Although considerable progress has been made in molecular design approaches for TADF materials, it still
Yuewei Zhang +8 more
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The increasing demand for high-performance organic light-emitting devices (OLEDs) based on thermally-activated delayed fluorescence (TADF) principle urgently requires to establish an efficient preparation strategy of high-performance TADF materials. Although considerable progress has been made in molecular design approaches for TADF materials, it still
Yuewei Zhang +8 more
openaire +1 more source
Chemical Communications, 2022
Ag(I)-promoted regioselective intramolecular radical nucleophilic addition/rearrangement of 2-aryl diazaboroles has been accomplished to construct phenazine structures, which is an umpolung strategy based on the classical electrophilic mechanism.
Huaxing Zhang +5 more
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Ag(I)-promoted regioselective intramolecular radical nucleophilic addition/rearrangement of 2-aryl diazaboroles has been accomplished to construct phenazine structures, which is an umpolung strategy based on the classical electrophilic mechanism.
Huaxing Zhang +5 more
openaire +2 more sources
Chemical Communications, 2012
Efficient thermally activated delayed fluorescence (TADF) was developed in a material based on a phenoxazine (PXZ) electron donor unit and a 2,4,6-triphenyl-1,3,5-triazine (TRZ) electron acceptor unit. An organic light-emitting diode containing this novel TADF emitter layer was fabricated and exhibited a maximum external quantum efficiency of 12.5 ...
Hiroyuki, Tanaka +3 more
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Efficient thermally activated delayed fluorescence (TADF) was developed in a material based on a phenoxazine (PXZ) electron donor unit and a 2,4,6-triphenyl-1,3,5-triazine (TRZ) electron acceptor unit. An organic light-emitting diode containing this novel TADF emitter layer was fabricated and exhibited a maximum external quantum efficiency of 12.5 ...
Hiroyuki, Tanaka +3 more
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Angewandte Chemie International Edition, 2019
AbstractCurrent research on thermally activated fluorescence (TADF) emitters is mainly based on the molecular levels, while the aggregation states of TADF emitters are to be explored deeply. Now two multifunctional emitters are reported with simultaneous TADF, aggregation induced emission (AIE), and multicolor mechanochromic luminescence (MCL) features.
Kailu Zheng +4 more
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AbstractCurrent research on thermally activated fluorescence (TADF) emitters is mainly based on the molecular levels, while the aggregation states of TADF emitters are to be explored deeply. Now two multifunctional emitters are reported with simultaneous TADF, aggregation induced emission (AIE), and multicolor mechanochromic luminescence (MCL) features.
Kailu Zheng +4 more
openaire +2 more sources
Angewandte Chemie
AbstractThe study of facile‐synthesis and low‐cost X‐ray scintillators with high light yield, low detection limit and high X‐ray imaging resolution plays a vital role in medical and industrial imaging fields. However, the optimal balance between X‐ray absorption, decay lifetime and excitonic utilization efficiency of scintillators to achieve high ...
Wen‐Fei Wang +8 more
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AbstractThe study of facile‐synthesis and low‐cost X‐ray scintillators with high light yield, low detection limit and high X‐ray imaging resolution plays a vital role in medical and industrial imaging fields. However, the optimal balance between X‐ray absorption, decay lifetime and excitonic utilization efficiency of scintillators to achieve high ...
Wen‐Fei Wang +8 more
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The Journal of Physical Chemistry A, 2018
The excited state properties of a series of binuclear NHetPHOS-Cu(I) complexes (NHetPHOS) have been investigated by means of density functional theory (DFT) and time-dependent DFT (TD-DFT). It is shown that experimental trends observed in powder, generally explored via S1 and T1 excited state energetics and S1 ⇔ T1 intersystem crossing (ISC) efficiency,
Ange Stoïanov +3 more
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The excited state properties of a series of binuclear NHetPHOS-Cu(I) complexes (NHetPHOS) have been investigated by means of density functional theory (DFT) and time-dependent DFT (TD-DFT). It is shown that experimental trends observed in powder, generally explored via S1 and T1 excited state energetics and S1 ⇔ T1 intersystem crossing (ISC) efficiency,
Ange Stoïanov +3 more
openaire +2 more sources