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A Carbon‐Induced Surface Reconstruction on an Operating Fischer–Tropsch Catalyst

open access: yesAngewandte Chemie International Edition, EarlyView.
It is widely believed that a cobalt Fischer–Tropsch catalyst initially undergoes an activity‐enhancing roughening, driven by the high chemical potential of carbon. In this operando STM and DFT study, we simulate such conditions. We show that, instead, a triangular stacking‐fault reconstruction may form, leaving the catalytic activity unchanged ...
Sebastian Kläger   +3 more
wiley   +1 more source

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