Results 81 to 90 of about 415,247 (217)

High Thermoelectric Performance in Low‐Cost Cu8SiSxSe6‐x Argyrodite

open access: yesAdvanced Functional Materials, EarlyView.
This study discovers the great potential of Cu8SiSxSe6‐x argyrodites as new, low‐cost, Te‐free thermoelectric materials. The proposed defect scheme suppresses the phase transition, enhances the weighted mobility and optimizes the grain boundary contacts.
Taras Parashchuk   +7 more
wiley   +1 more source

Supercompliant Lattice Boosts n‐type AgSbTe2 Thermoelectrics

open access: yesAdvanced Functional Materials, EarlyView.
The supercompliant lattice design enables the first realization of n‐type electrical transport in AgSbTe2 by overcoming intrinsic electron‐killer defects and exceeding the doping limits imposed by the conventional Hume–Rothery rule. Accordingly, the best performance n‐type Ag0.8Na0.3Sb0.6Bi0.4Te2 sample achieves a low κ of 0.27 W·m−1·K−1 that ...
Ruoyan Li   +15 more
wiley   +1 more source

Coupling Interfacial Redox‐Reactions with In Situ Proton Generation for the Photoelectrochemical Separation of Rare‐Earth Elements

open access: yesAdvanced Functional Materials, EarlyView.
To enhance the sustainability of electrochemical separations for resource recovery, a photoelectrochemical ion recovery system is developed that utilizes renewable solar energy. A composite integrating titianium dioxide nanorods and a redox‐copolymer enables spontaneous cation adsorption and light‐activated redox reactions for regeneration, thus ...
Ki‐Hyun Cho   +3 more
wiley   +1 more source

Unit Disk Cover Problem

open access: yes, 2012
Given a set ${\cal D}$ of unit disks in the Euclidean plane, we consider (i) the {\it discrete unit disk cover} (DUDC) problem and (ii) the {\it rectangular region cover} (RRC) problem. In the DUDC problem, for a given set ${\cal P}$ of points the objective is to select minimum cardinality subset ${\cal D}^* \subseteq {\cal D}$ such that each point in $
Acharyya, Rashmisnata   +2 more
openaire   +2 more sources

Transient Stiffness Patterning in Hydrogels Driven by Dissipative Mechanochemical Coupling

open access: yesAdvanced Functional Materials, EarlyView.
Force‐induced disulfide bond rupture in a polymer‐based hydrogel, coupled with chemical or electrochemical reoxidation, leads to the transient modulation of the hydrogel's stiffness properties. High spatiotemporal control is achieved by this dissipative process, enabling the development of out‐of‐equilibrium stiffness patterns and transient, dose ...
Roberto Baretta   +2 more
wiley   +1 more source

Deciphering a New Electrolyte Formulation for Intelligent Modulation of Thermal Runaway to Improve the Safety of Lithium‐Ion Batteries

open access: yesAdvanced Functional Materials, EarlyView.
Diels‐Alder clicks chemistry addresses thermal runaway in lithium‐ion batteries. A thermoresponsive electrolyte with lithium salt in vinylene carbonate (VC) and 2,5‐dimethylfuran (DMFu) operates at room temperature but undergoes Diels‐Alder reactions at high temperatures, enabling a two‐step safety mechanism: a warning phase at ≈100 °C and complete ...
Arnab Ghosh   +9 more
wiley   +1 more source

Atomic Size Misfit for Electrocatalytic Small Molecule Activation

open access: yesAdvanced Functional Materials, EarlyView.
This review explores the application and mechanisms of atomic size misfit in catalysis for small molecule activation, focusing on how structural defects and electronic properties can effectively lower the energy barriers of chemical bonds in molecules like H2O, CO2, and N2.
Ping Hong   +3 more
wiley   +1 more source

Decoding the Structure of Benzodithiophene Polymers for High‐Efficiency Organic Solar Cells

open access: yesAdvanced Functional Materials, EarlyView.
This study reveals a unique solid mesophase in top‐performing benzodithiophene‐based polymers for solar cells, comprising stacked solid‐like and liquid‐like layers. Combining nanoscale fibrillar domains with amorphous regions, it introduces a new structural paradigm.
Matteo Sanviti   +16 more
wiley   +1 more source

Ultrahigh‐resolution (λ/10) Femtosecond Laser Writing of Polymer‐Encapsulated Multicolor Perovskite Patterns Beyond the Diffraction Limit

open access: yesAdvanced Functional Materials, EarlyView.
Fabrication of in situ polymer‐encapsulated stable perovskite patterns of arbitrary shapes and pixel arrays with a resolution of 80 nm is reported by the femtosecond (fs) laser (800 nm) super‐resolution writing technique. The two‐photon absorption‐induced laser ablation is attributed to the achieved feature sizes as small as λ/10.
Xuebing Wen   +8 more
wiley   +1 more source

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