Results 91 to 100 of about 50,919 (218)

High‐Mobility Chalcogenophene‐Engineered Diketopyrrolopyrrole Mixed Ionic‐Electronic Conductors With Doping Tolerance for Low‐Power Organic Electrochemical Transistors

Advanced Materials, EarlyView.
Chalcogen substitution emerges as a powerful strategy for designing high‐performance OMIECs. In aliphatic–glycol side chain diketopyrrolopyrrole polymers, biselenophene incorporation promotes a planar, polarizable, and doping‐tolerant quinoidal framework, enabling PDPP‐4EG‐Se2 to combine high hole mobility, large µC*, enhanced operational stability ...
Shinbee Oh, Tae Hoon Kim, Dahyun Jeong, Ji Hwan Kim, Seungjin Lee, Tan Ngoc‐Lan Phan, Alexander Tipan‐Quishpe, Myung‐Han Yoon, Keehoon Kang, Bumjoon J. Kim   +9 more
wiley   +1 more source

Charge Storage and Dark Photocatalysis in Multivariate Ti‐Based Metal‐Organic Frameworks

Advanced Materials, EarlyView.
The mixed‐linker series of the titanium‐based metal–organic framework COK‐47 enables systematic tuning of photoresponsiveness and (dark) photocatalytic activity, deepening our understanding of structure‐property‐function relationships. Tailored metal‐to‐ligand charge transfer between the secondary building units (metal‐oxo layers and organic linkers ...
Julia E. Knapp, Bibhuti Bhusan Rath, Borja Ortín‐Rubio, Lukas Bauder, Kristina Gjorgjevikj, Saunak Das, Mariia Ferree, Frédéric Laquai, Lorenzo Tesi, Bettina Baumgartner, Simon Krause, Bettina V. Lotsch   +11 more
wiley   +1 more source

In Situ Formation of a Highly Selective Nickel Single Atom Catalyst for Electrochemical CO2 Reduction to CO

Advanced Materials, EarlyView.
Development of a novel method for synthesizing Ni single atom catalysts for highly selective electrochemical CO2 reduction in situ. This catalyst achieves 100% selectivity for CO and is formed in an industrially relevant cell architecture. Using post‐mortem XRD, STEM, and EDS and operando XAS, the identity of the active site and the mechanism behind ...
Ian Street, Venkata Sai Sriram Mosali, Noah Sandberg, Fengyuan Shi, Deborah Myers, William E. Mustain   +5 more
wiley   +1 more source

Pulsed Oxidative–Reductive Electrolysis Over Dual Cu and Co Single‐Atom Sites for Urea Electrosynthesis

Advanced Materials, EarlyView.
Alternating oxidative–reductive pulses synchronize CO2‐derived *CO and NH3‐derived *NHx intermediates over dual Cu and Co single‐atom sites, enabling urea and ethyl urea formation with a total C─N Faradaic efficiency of 42 ± 4%. In situ spectroscopy and theoretical calculations elucidate complementary Cu and Co functions, while oxidative controls ...
Putri Ramadhany, Peiqi Qiu, Thành Trần‐Phú, Denny Gunawan, Bernt Johannessen, Rosalie K. Hocking, Yan Jiao, Rose Amal, Rahman Daiyan   +8 more
wiley   +1 more source

Directional Confinement Governed Ion Transport for Efficient Actuation

Advanced Materials, EarlyView.
Structural anisotropy provides an effective means to regulate ion transport in polymer electrolytes. Directionally aligned channels formed by freeze‐drying provide continuous pathways for ion migration, enhancing ion mobility and simultaneously improving the strain and blocking force of ionic actuators.
Yufei Zhang, Qiuchun Lu, Adit Gupta, Sen Wang, Xueyang Wang, Jian Yu, Xuanyi Hu, Daniel Mandler, Pooi See Lee   +8 more
wiley   +1 more source

Integrated system for electrolyte recovery, product separation, and CO2 capture in CO2 reduction

Nature Communications
Challenges in CO2 capture, CO2 crossover, product separation, and electrolyte recovery hinder electrocatalytic CO2 reduction (CO2R). Here, we present an integrated electrochemical recovery and separation system (ERSS) with an ion separation module (ISM ...
Peng Wang, An Pei, Zhaoxi Chen, Peilin Sun, Chengyi Hu, Xue Wang, Nanfeng Zheng, Guangxu Chen   +7 more
doaj   +1 more source

Turning Nd‐Fe‐B Swarf Into High‐Value Bulk Feedstocks via Sustainable Hydrogen Plasma: From Rare‐Earth Oxides to Metals and Hydrides

Advanced Materials, EarlyView.
Oxidized Nd‐Fe‐B magnet swarf is transformed into valuable bulk feedstock through a single‐step hydrogen plasma process. The reaction converts complex rare‐earth‐containing waste into separated metallic, oxide, and hydride fractions without acid leaching.
Naritai Chimed, Oliver Diehl, Ömer K. Büyükuslu, J. Manoj Prabhakar, Dennis Klapproth, Patricia Jovičević‐Klug, Jürgen Gassmann, Dierk Raabe, Tim M. Schwarz, Matic Jovičević‐Klug   +9 more
wiley   +1 more source

Advances in Bio‐Integrated Edge Computing Systems for Smart and Connected Health

Advanced Materials, EarlyView.
This review explores advances in bio‐integrated edge computing for healthcare, focusing on co‐designing computing, sensing, and energy strategies to overcome integration and power challenges for optimized, decentralized operation. ABSTRACT Recent advances in bio‐integrated healthcare technologies have enabled continuous, high‐resolution monitoring and ...
Gyuwon Kim, Seungwon Yoo, Tae Woog Kang, Yunuo Huang, Woon‐Hong Yeo   +4 more
wiley   +1 more source

A Simple Descriptor for Solid‐State Ionic Conductors Across Chemistries

Advanced Materials, EarlyView.
Researchers develop a simple and transferable descriptor, distance contraction, for solid‐state ion migration across Li‐, Na‐, K‐, and Mg‐ion conductors and diverse anion chemistries. By capturing the maximum local contraction experienced by the migrating ion, the descriptor enables rapid materials screening and unifies diverse ion‐transport mechanisms.
Ramanuja Srinivasan Saravanan, Charles E. Schwarz, Felix Adams, Kiyan Amirian, Yifei Mo   +4 more
wiley   +1 more source