Results 41 to 50 of about 471 (187)

Conformally Perforated Shellular Metamaterials with Tunable Thermomechanical and Acoustic Properties

Advanced Functional Materials, EarlyView.
This study introduces Conformally Perforated Shellular Metamaterials (CPSMs), which overcome TPMS design limitations by mapping 2D cellular layouts onto 3D surfaces. CPSMs exhibit enhanced elastic stiffness, thermal conductivity, and acoustic performance compared to intact P‐type shellulars, demonstrating their potential as multifunctional ...
Benyamin Shahryari, Armin Mirabolghasemi, Shahin Eskandari, Xin Chen, Jean‐François Deü, Roger Ohayon, Atef Mohany, Alex Kalamkarov, Abdolhamid Akbarzadeh   +8 more
wiley   +1 more source

Bridging Theory and Experiment: Machine Learning Potential‐Driven Insights into pH‐Dependent CO₂ Reduction on Sn‐Based Catalysts

Advanced Functional Materials, EarlyView.
Machine learning potential (MLP) enables large‐scale molecular dynamics (MD) simulations, uncovering dynamic surface reconstruction of SnO₂ and SnS₂ under CO₂ reduction reaction condition. The negative dipole moments upon *OCHO adsorption are the primary factors driving the leftward shift of the volcano plot.
Yuhang Wang, Zelin Wu, Yingfang Jiang, Di Zhang, Qiang Wang, Congwei Wang, Huihui Li, Xue Jia, Jun Fan, Hao Li   +9 more
wiley   +1 more source

Multifunctional Polyfluoride Ionogel‐Encapsulated Lithium Anodes for Durable and Safe Pouch Cells under Harsh Conditions

Advanced Functional Materials, EarlyView.
In this work, it is developed a multifunctional polyfluoride ionogel via in situ thermal polymerization to encapsulate lithium metal anodes, integrating flame‐retardant capability, hydrophobicity, dynamic self‐healing behavior, and high ionic conductivity.
Ting Li, Anjun Hu, Yuanjian Li, Borui Yang, Kun Li, Kai Chen, Jingyun Jiang, Fei Li, Zhi Wei Seh, Jian Wang, Jianping Long   +10 more
wiley   +1 more source

Covalent Adaptable Networks with Associative Siloxane Exchange Enabled by Amide‐Based Internal Catalysis: Designing for Reprocessability and Extrudability by Increasing the Cross‐Link Density

Advanced Functional Materials, EarlyView.
Internally catalyzed siloxane dynamic chemistry is demonstrated resulting from amides covalently linked through alkyl chains to siloxanes. The alkyl length in the siloxane‐containing monomer tunes the network cross‐link density. Siloxane exchange dynamics are faster with increasing cross‐link density, because associative exchange is second order in ...
Nathan S. Purwanto, Tong Wang, Xiaoyang Liu, Linda J. Broadbelt, Tapas Debsharma, John M. Torkelson   +5 more
wiley   +1 more source

Highly Sensitive Electrochemical Biosensor Based on Hairy Particles with Controllable High Enzyme Loading and Activity

Advanced Functional Materials, EarlyView.
For the first time, a highly sensitive electrochemical biosensor based on SiO2‐based hairy particles with a grafted PDMAEMA polymer brush containing a quantifiable and large amount of immobilized Laccase is reported. The fabricated biosensor exhibits a sensitivity of 0.14 A·m⁻¹, a limit of detection (LOD) of 0.1 µm, and a detection range of 0.3–750 µm,
Pavel Milkin, Anila Antony, Hongtao Cai, Antonia Debevc, Ceyda Topal, Anne Linhardt, Alla Synytska, Leonid Ionov   +7 more
wiley   +1 more source

Tailored Polymer‐Based SEI via iCVD for Stable Zinc Metal Anodes in Aqueous Batteries through Modulation of Hydrophilicity and Elasticity to Inhibit Hydrogen Evolution Reactions

Advanced Functional Materials, EarlyView.
A stretchable and superhydrophobic pF1V1 polymer layer is conformally coated on Zn metal via iCVD, forming a water‐repelling interphase that inhibits the hydrogen evolution reaction. This tailored interface maintains excellent electrolyte compatibility while suppressing dendrite growth, thereby enhancing the long‐term electrochemical stability of Zn ...
Jaeyeon Lee, Moonwon Lee, Boyeon Kim, Hyunjin Jung, Kanghoon Yim, Myunghyun Ryu, Gi Su Doo, Jae‐Hak Choi, Jiyun Heo, Sung Gap Im, Kyu‐Nam Jung, Myung Seok Oh, Jinhong Lee   +12 more
wiley   +1 more source

Cu2O/Cu Chiral Catalysts for Highly Selective Solar‐Assisted CO2‐to‐CO Electroreduction

Advanced Functional Materials, EarlyView.
To address the poor target‐product selectivity of the eCO2RR, breakthrough approaches based on the chiral‐induced spin selectivity phenomenon enhance the Faradaic efficiency (FE) for target hydrocarbons, such as CO. To induce this spin polarization strategy in Cu2O/Cu catalysts, it is proposed using amine‐based intermediate organic molecules with ...
Hyungsoo Lee, Young Sun Park, Eunji Kwon, Chang‐Seop Jeong, Juwon Yun, Subin Moon, Soobin Lee, Jun Hwan Kim, Donghyun Kim, Wooyong Jeong, Jaehyun Son, Jihwon Park, Seungho Yu, Jooho Moon   +13 more
wiley   +1 more source

Additively Manufactured 3D Auxetic Metamaterials for Structurally Guided Capacitive and Resistive Tactile Sensing

Advanced Functional Materials, EarlyView.
A 3D‐architected auxetic metamaterial is used to construct capacitive and resistive tactile sensors via digital light processing‐based additive manufacturing. The inward deformation of the proposed structure under compression amplifies local strain, enhancing sensing performance.
Mingyu Kang, Hong‐Gap Choi, Keun Park, Soonjae Pyo   +3 more
wiley   +1 more source

Aerosol Jet Printed MXene Microsupercapacitors for Flexible and Washable Textile Energy Storage

Advanced Functional Materials, EarlyView.
This study introduces a novel approach using aerosol jet printing to fabricate e‐textiles with additive‐free aqueous Ti3C2Tx MXene inks. The flexible electrodes, systematically explored on cotton, polycotton, and polyester, exhibit remarkable areal capacitances of up to 4.4 F cm−2, achieving superior high‐rate performance, capacitance retention, and ...
Anastasiia Shandra, Ke Li, Dahnan Spurling, Oskar Ronan, Valeria Nicolosi   +4 more
wiley   +1 more source

Enhancing Mechanical Deformability of Rigid Conjugated Polymers through Functional Additive‐Induced Persistence Length Modulation

Advanced Functional Materials, EarlyView.
This study demonstrates a molecular strategy to enhance the stretchability of conjugated polymers by incorporating plasticizing molecular additives (PMAs). PMAs reduce the persistence length and promote chain entanglement, enabling deformable thin films with preserved electrical performance. A systematic analysis combining rheology, neutron scattering,
Sein Chung, Seung Hyun Kim, Sanghyo Kim, Eunsol Ok, Byeong Jin Kim, Jimin Kim, Jiyeong Shin, Taehun Chung, Jong Dae Jang, Siyoung Lee, Boseok Kang, Kilwon Cho   +11 more
wiley   +1 more source