Results 141 to 150 of about 233,942 (302)

Balancing Electrons to Break the Activity‐Selectivity Trade‐Off in H2O2 Electrosynthesis

open access: yesAdvanced Functional Materials, EarlyView.
Carrier‐concentration balancing in CuS is achieved by coupling cobalt dopants with cobalt vacancies, converting CuS from p‐ to n‐type to accelerate 2e− ORR while withdrawing excess carriers to optimize *OOH binding for H2O2 desorption. The catalyst reaches 8.14 mol g−1 h−1 with >84% selectivity in 1.0 M KOH and drives robust electro‐Fenton dye ...
Hangning Liu   +11 more
wiley   +1 more source

Engineering Hydrogen‐Down Water Configurations for Ampere‐Level Electrochemical CO2 Reduction to Formate

open access: yesAdvanced Functional Materials, EarlyView.
Electrochemical CO2 reduction (ECR) to formate is a promising route for sustainable chemical production. Herein, we report the synthesis catalysed byBi‐HfO2@C. The AIMD simulations, DFT calculations, and in situ SEIRAS measurements show that the modification of HfO2 on the Bi surface steers the interfacial water to adopt a favorable hydrogen‐down (OH2↓)
Xiao‐Dong Guo   +7 more
wiley   +1 more source

Giant Intrinsic Chirality Amplification of Aqueous Lead Halide Perovskite Nanocrystals via H‐Bond Driven Self‐Assembly Superstructures

open access: yesAdvanced Functional Materials, EarlyView.
Water‐assisted monoclinic CsPbBr3 transformation strategy is applied for synthesizing aqueous CsPbBr3/CsPb2Br5 nanocrystals with superior water‐repellent and excellent optical property. Low temperature enhanced hydrogen bonding network self‐assembled CsPbBr3/CsPb2Br5 nanocrystals into asymmetric superstructures, which exhibit notable circularly ...
Mei Huang   +7 more
wiley   +1 more source

Observation of Two‐Photon Resonant Raman Scattering via the Biexciton Level in Two‐Dimensional Halide Perovskite (C6H5C2H4NH3)2PbI4

open access: yesAdvanced Functional Materials, EarlyView.
Efficient two‐photon resonant Raman scattering (TRRS) is observed in the layered perovskite (PEA)2PbI4, with the biexciton level acting as an intermediate state. TRRS undergoes two‐photon frequency shift upon input frequency tuning, persists up to 90 K, and shows clear threshold behavior and polarization selection rules.
Seung Han Shin   +7 more
wiley   +1 more source

Quantification of Soil Organic Carbon by Shifted-Excitation Raman Difference Spectroscopy with Machine Learning and Common Mode Rejection. [PDF]

open access: yesAnal Chem
Brown GW   +9 more
europepmc   +1 more source

Graphene Nanosheet‐Based Mixed Proton‐Electron Conducting Membranes for Efficient Hydrogen Purification

open access: yesAdvanced Functional Materials, EarlyView.
A monolayer graphene/phosphoric‐acid mixed proton‐electron conducting membrane combines proton‐conducting nanoconfined acid channels with electron‐conducting graphene nanosheets for efficient high‐temperature hydrogen purification. The membrane achieves nearly 100% H2/CO2 selectivity and 69 GPU hydrogen permeance at 250°C, arising from synergistic ...
Kaiqiang He   +8 more
wiley   +1 more source

3D‐Printed Hygroscopic Polymer Networks for High‐Humidity Triboelectric Nanogenerators to Wirelessly Power Implantable Electronic Devices‐ A Conceptual Pathway

open access: yesAdvanced Functional Materials, EarlyView.
This work develops 3D‐printable tribopolymer networks that can enhance triboelectric performance under high humidity environments. Polar hydrophilic functional groups and incorporation of zwitterionic monomers promote bound‐water–dominated interfacial polarization thereby increasing electrical outputs.
Linguangze Zhuo   +8 more
wiley   +1 more source

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