Results 91 to 100 of about 53,720 (260)

Mechanistic Insights Into Instability From Single Void Dynamics at the Lithium Metal‐Solid Electrolyte Interface

Advanced Science, EarlyView.
Void morphology at the lithium metal‐solid electrolyte contact governs electrochemical contact stability in all‐solid‐state batteries. This work resolves the competing roles of electrochemical reaction, bulk vacancy diffusion, and distinct surface diffusion pathways in dictating the size and morphology evolution of a single void and its transition to a
Sourim Banerjee, Bairav S. Vishnugopi, Guang Lin, Partha P. Mukherjee   +3 more
wiley   +1 more source

Vacuum‐Induced Surface Reconstruction of Mn–Ce Oxides for Low‐Temperature Coupled Redox Catalysis

Angewandte Chemie, EarlyView.
Near‐surface reconstruction enhances low‐temperature redox catalysis in Mn–Ce mixed oxides. Sequential vacuum annealing and reduced‐pressure O2 treatment enrich Mn near the surface while preserving the CeO2 fluorite framework, promoting interfacial electron redistribution, oxygen activation, and redox cycling.
Yong Yin, Yide Jiang, Zichen Xu, Min Liu, Emiliano Cortés, Yifei Sun   +5 more
wiley   +2 more sources

Electronic‐State Programming of Ultrasmall CeO2 Switches H2O2 Activation From Radical to Bio‐Inspired Nonradical 1O2 Generation for Combating Antibiotic Resistance

Advanced Science, EarlyView.
A scalable synthesis of carbon‐supported ultrasmall CeO2 nanoparticles with precisely tunable Ce electron density is reported. Electron‐lean Ce sites activate H2O2 exclusively via a nonradical pathway, enabling efficient HOBr and 1O2 production analogous to bromoperoxidase for contaminant and antibiotic resistance removal.
Bo Yuan, Xinyu Wu, Yin‐Song Liao, Chao Zhao, Zhanping Xiao, Wanqing Dai, Jyh‐Pin Chou, Wenchao Peng, Jian Lin Chen, Pi‐Tai Chou, Yung‐Kang Peng   +10 more
wiley   +1 more source

Elucidating Photo‐Kinetic Control in Photothermal Reverse Water‐Gas Shift Reaction

Angewandte Chemie, EarlyView.
Light directly regulates the rate‐determining step (RDS) in photothermal catalysis. In a Mars–van Krevelen (MvK)‐type reverse water‐gas shift (RWGS) reaction over In‐doped MoO2, light shifts the RDS from the H2‐related reduction half‐reaction to the CO2‐related oxidation half‐reaction, enhancing catalytic activity and lowering the apparent activation ...
Junchuan Sun, Rui Song, Chang Xu, Xue Ding, Wanguo Gao, Athanasios A. Tountas, Zhe Lu, Jiakun Wang, Zeshu Zhang, Xiaolu Zhuo, Yingfang Yao, Zhigang Zou, Geoffrey A. Ozin, Lu Wang   +13 more
wiley   +2 more sources

Subsurface State Bilayer in Tetragonal Ferroelectric BaTiO3

Advanced Materials Interfaces
The interface is an issue in the ferroelectric field effect transistor. In this work, the study presents a combined characterization of the subsurface structure and the electric polarization of (001)‐oriented and poled BaTiO3 crystal sheets.
Junhao Chen, Xin Su, Tao Yuan, Wenbin Tang, Shicheng Ding, Yan Shi, Fangming Li, Kai Chen, Yang Yu, Hongchao Zhang, Siyuan Zhu, Guoliang Yuan, Jian Lu   +12 more
doaj   +1 more source

Advancing Energy Materials by In Situ Atomic Scale Methods

Advanced Energy Materials, Volume 15, Issue 11, March 18, 2025.
Progress in in situ atomic scale methods leads to an improved understanding of new and advanced energy materials, where a local understanding of complex, inhomogeneous systems or interfaces down to the atomic scale and quantum level is required. Topics from photovoltaics, dissipation losses, phase transitions, and chemical energy conversion are ...
Christian Jooss, Michael Seibt, Martin Wenderoth, Oliver Bünermann, Ole Bunjes, Till Domröse, Christian Eckel, Francesca Falorsi, Christoph Flathmann, Monica Kolek Martinez de Azagra, Matthias Krüger, Jonas Lindner, Tobias Meyer, Claus Ropers, Ulrich Ross, Kai Rossnagel, Sreeju Sreekantan Nair Lalithambika, Simone Techert, Georg A. Traeger, Cynthia Volkert, R. Thomas Weitz, Alec M. Wodtke   +21 more
wiley   +1 more source

Decoupling Chemical and Mechanical Contributions to Capacity Fading in Ni‐Rich Cathodes for Sulfide‐Based All‐Solid‐State Batteries

Advanced Energy Materials, EarlyView.
Ni‐rich cathodes in sulfide‐based ASSBs undergo intertwined (electro)chemical and mechanical degradation. Here, a new diagnostic framework is presented to decouple each contribution by partitioning capacity fading into charge and discharge fading.
Jangwhan Seok, Chanyou Chung, Hyunbeom Lee, Subin Ahn, Seongeun Lee, Sangbin Park, Sunhyun Hwang, Jaeyoung Kim, Jeonghyun Seo, Sungwoo Noh, Juyeong Seong, Sangheon Lee, Won‐Sub Yoon   +12 more
wiley   +1 more source

Enabling Fast Charging of Lithium‐Ion Batteries With Regioisomeric Nitrile Additives for Interphase Regulation

Angewandte Chemie, EarlyView.
Fast charging and low‐temperature operation of lithium‐ion batteries (LIBs) are achieved by incorporating only 0.5 wt.% of a nitrile‐based additive into the commercial LP57 electrolyte. The additive enhances Li+ transport, stabilizes the solid‐electrolyte and cathode‐electrolyte interphases (SEI and CEI), and suppresses lithium plating.
Chen Liu, Zehao Cui, Arumugam Manthiram
wiley   +2 more sources

Leveraging Neural Operator and Sliding Window Technique for Enhanced Subsurface Soil Moisture Imputation Under Diverse Precipitation Scenarios

Journal of Geophysical Research: Machine Learning and Computation
Environmental monitoring and decision‐making are sometimes hampered by missing sensor data, particularly in soil moisture (SM) records that underpin hydrological modeling, agricultural management, and climate studies.
Abhilash Singh, Vidhi Singh, Kumar Gaurav   +2 more
doaj   +1 more source

Dry‑Contact Trimming for All‑Perovskite Tandem Solar Cells via Solid‑Solution Homogenization

Advanced Energy Materials, EarlyView.
Narrow‐bandgap Sn–Pb perovskites are promising bottom absorbers for all‐perovskite tandems but suffer from Sn‐rich surfaces and depth‐dependent lattice/compositional inhomogeneity. Layered‐perovskite‐assisted dry‐contact trimming removes Sn‐rich surface species and reconfigures the Sn–Pb absorber, enabling efficient charge collection, reduced voltage ...
Woocheol Han, Hyojin Hong, Chan Young Kim, Chan Ho Shin, Sung Yong Kim, So Eun Shin, Minhyeok Park, Giseon Yu, Sohyun Kang, Seungmin Lee, Jun Hong Noh   +10 more
wiley   +1 more source