Effect of Stratosphere-Troposphere Exchange on the Future Tropospheric Ozone Trend [PDF]
This paper investigates the impact of circulation changes in a changed climate on the exchange of ozone between the stratosphere and the troposphere. We have identified an increase in the net transport of ozone into the troposphere in the future climate of 37%, although a decreased ozone lifetime means that the overall tropospheric burden decreases ...
Michael Sanderson +2 more
exaly +4 more sources
Effects of stratosphere‐troposphere chemistry coupling on tropospheric ozone [PDF]
A new, computationally efficient coupled stratosphere‐troposphere chemistry‐climate model (S/T‐CCM) has been developed based on three well‐documented components: a 64‐level general circulation model from the UK Met Office Unified Model, the tropospheric chemistry transport model (STOCHEM), and the UMSLIMCAT stratospheric chemistry module.
Tian, Wenshou +7 more
openaire +3 more sources
A model study Of chemistry and transport in the Arctic troposphere [PDF]
In this thesis the TOMCAT chemical transport model is used to investigate the processes which control the concentrations of CO and O3 in the Arctic troposphere. Particular focus is on understanding the main sources of CO, O3 and NOy species in the Arctic,
Monks, Sarah Anne
core +6 more sources
Atmospheric photooxidation and ozonolysis of sabinene: reaction rate coefficients, product yields, and chemical budget of radicals [PDF]
The oxidation of sabinene by the hydroxyl radical (OH) and ozone (O3) was investigated under atmospherically relevant conditions in the atmospheric simulation chamber SAPHIR (Simulation of Atmospheric Photochemistry In a Large Reaction Chamber) at ...
J. Y. S. Pang +12 more
doaj +1 more source
Air quality observations onboard commercial and targeted Zeppelin flights in Germany – a platform for high-resolution trace-gas and aerosol measurements within the planetary boundary layer [PDF]
A Zeppelin airship was used as a platform for in situ measurements of greenhouse gases and short-lived air pollutants within the planetary boundary layer (PBL) in Germany.
R. Tillmann +13 more
doaj +1 more source
Experimental chemical budgets of OH, HO2, and RO2 radicals in rural air in western Germany during the JULIAC campaign 2019 [PDF]
Photochemical processes in ambient air were studied using the atmospheric simulation chamber SAPHIR at Forschungszentrum Jülich, Germany. Ambient air was continuously drawn into the chamber through a 50 m high inlet line and passed through the chamber ...
C. Cho +20 more
doaj +1 more source
Atmospheric photo-oxidation of myrcene: OH reaction rate constant, gas-phase oxidation products and radical budgets [PDF]
The photo-oxidation of myrcene, a monoterpene species emitted by plants, was investigated at atmospheric conditions in the outdoor simulation chamber SAPHIR (Simulation of Atmospheric PHotochemistry In a Large Reaction Chamber). The chemical structure of
Z. Tan +20 more
doaj +1 more source
Electrochemical sensors on board a Zeppelin NT: in-flight evaluation of low-cost trace gas measurements [PDF]
In this work, we used a Zeppelin NT equipped with six sensor setups, each composed of four different low-cost electrochemical sensors (ECSs) to measure nitrogen oxides (NO and NO2), carbon monoxide, and Ox (NO2+O3) in Germany.
T. Schuldt +7 more
doaj +1 more source
Reactive Nitrogen in the Tropical Troposphere [PDF]
The aim of this project was to calibrate a thermal-decomposition chemiluminescence (TD-Chem) instrument, capable of measuring the composition of the reactive nitrogen pool at the Cape Verde Atmospheric Observatory (CVAO) in the remote tropical ...
Manning, William D
core +5 more sources
Photooxidation of pinonaldehyde at ambient conditions investigated in the atmospheric simulation chamber SAPHIR [PDF]
The photooxidation of pinonaldehyde, one product of the α-pinene degradation, was investigated in the atmospheric simulation chamber SAPHIR under natural sunlight at low NO concentrations (<0.2 ppbv) with and without an added hydroxyl radical ...
M. Rolletter +16 more
doaj +1 more source

